THz-Enhanced DC Ultrafast Electron Diffractometer

Author:

Zhang Dongfang12ORCID,Kroh Tobias13ORCID,Ritzkowsky Felix13ORCID,Rohwer Timm1,Fakhari Moein13,Cankaya Huseyin13ORCID,Calendron Anne-Laure1,Matlis Nicholas H.1,Kärtner Franz X.13ORCID

Affiliation:

1. Center for Free-Electron Laser Science, Deutsches Elektronen Synchrotron, Notkestrasse 85, 22607 Hamburg, Germany

2. Collaborative Innovation Center for IFSA, School of Physics and Astronomy, Shanghai Jiao Tong University, 200240 Shanghai, China

3. Department of Physics and The Hamburg Centre for Ultrafast Imaging, Universität Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany

Abstract

Terahertz- (THz-) based electron manipulation has recently been shown to hold tremendous promise as a technology for manipulating and driving the next generation of compact ultrafast electron sources. Here, we demonstrate an ultrafast electron diffractometer with THz-driven pulse compression. The electron bunches from a conventional DC gun are compressed by a factor of 10 and reach a duration of ~180 fs (FWHM) with 10,000 electrons/pulse at a 1 kHz repetition rate. The resulting ultrafast electron source is used in a proof-of-principle experiment to probe the photoinduced dynamics of single-crystal silicon. The THz-compressed electron beams produce high-quality diffraction patterns and enable the observation of the ultrafast structural dynamics with improved time resolution. These results validate the maturity of THz-driven ultrafast electron sources for use in precision applications.

Funder

Gordon and Betty Moore Foundation

Publisher

American Association for the Advancement of Science (AAAS)

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