An X-Ray Tomography Based Lattice Boltzmann Simulation Study on Gas Diffusion Layers of Polymer Electrolyte Fuel Cells

Author:

Rama Pratap1,Liu Yu1,Chen Rui1,Ostadi Hossein2,Jiang Kyle2,Zhang Xiaoxian3,Fisher Rosemary4,Jeschke Michael4

Affiliation:

1. Department of Aeronautical and Automotive Engineering, Loughborough University, LE11 3TU, UK

2. School of Mechanical and Manufacturing Engineering, Centre for Biomedical and Nanotechnology, University of Birmingham, B15 2TT, UK

3. Department of Engineering, University of Liverpool, L69 3GQ, UK

4. Technical Fibre Products Limited, Kendal, LA9 6PZ, UK

Abstract

This work reports a feasibility study into the combined full morphological reconstruction of fuel cell structures using X-ray computed micro- and nanotomography and lattice Boltzmann modeling to simulate fluid flow at pore scale in porous materials. This work provides a description of how the two techniques have been adapted to simulate gas movement through a carbon paper gas diffusion layer (GDL). The validation work demonstrates that the difference between the simulated and measured absolute permeability of air is 3%. The current study elucidates the potential to enable improvements in GDL design, material composition, and cell design to be realized through a greater understanding of the nano- and microscale transport processes occurring within the polymer electrolyte fuel cell.

Publisher

ASME International

Subject

Mechanical Engineering,Mechanics of Materials,Energy Engineering and Power Technology,Renewable Energy, Sustainability and the Environment,Electronic, Optical and Magnetic Materials

Reference39 articles.

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2. Ji, C., and Fly, G. W., “Increasing the Hydrophilicity of Carbon Fiber Paper by Electropolymerization,” U.S. Patent No. 7,250,189.

3. Diffusion Layer Parameters Influencing Optimal Fuel Cell Performance;Jordan;J. Power Sources

4. Development and Electrochemical Studies of Gas Diffusion Electrodes for Polymer Electrolyte Fuel Cells;Paganin;J. Appl. Electrochem.

5. Influence of the PTFE Content in the Diffusion Layer of Low-Pt Loading Electrodes for Polymer Electrolyte Fuel Cells;Giorgi;Electrochim. Acta

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