Numerical Modeling of Polymer Electrolyte Fuel Cells With Analytical and Experimental Validation-Reference-Cited by-同舟云学术

Numerical Modeling of Polymer Electrolyte Fuel Cells With Analytical and Experimental Validation

Published:2019-01-22 Issue:3 Volume:16 Page:
ISSN:2381-6872
Container-title:Journal of Electrochemical Energy Conversion and Storage
language:en
Short-container-title:

Author:

Zhang S.¹,Reimer U.¹,Rahim Y.¹,Beale S. B.²³,Lehnert W.⁴⁵⁶

Affiliation:

1. Forschungszentrum Jülich GmbH IEK-3, Electrochemical Process Engineering, Jülich 52425, Germany e-mail:

2. Fellow ASME Forschungszentrum Jülich GmbH IEK-3, Electrochemical Process Engineering, Jülich 52425, Germany;

3. Mechanical and Materials Engineering, Queen's University, Kingston K7L 3N6, ON, Canada e-mail:

4. Forschungszentrum Jülich GmbH IEK-3, Electrochemical Process Engineering, Jülich 52425, Germany;

5. Modeling in Electrochemical Process Engineering, RWTH Aachen University, Aachen 52056, Germany;

6. JARA-HPC, Jülich 52425, Germany e-mail:

Abstract

A computational fluid dynamics model for high-temperature polymer electrolyte fuel cells (PEFC) is developed. This allows for three-dimensional (3D) transport-coupled calculations to be conducted. All major transport phenomena and electrochemical processes are taken into consideration. Verification of the present model is achieved by comparison with current density and oxygen concentration distributions along a one-dimensional (1D) channel. Validation is achieved by comparison with polarization curves from experimental data gathered in-house. Deviations between experimental and numerical results are minor. Internal transport phenomena are also analyzed. Local variations of current density from under channel regions and under rib regions are displayed, as are oxygen mole fractions. The serpentine gas channels contribute positively to gas redistribution in the gas diffusion layers (GDLs) and channels.

Funder

Chinese Government Scholarship

Publisher

ASME International

Subject

Mechanical Engineering,Mechanics of Materials,Energy Engineering and Power Technology,Renewable Energy, Sustainability and the Environment,Electronic, Optical and Magnetic Materials

Link

http://asmedigitalcollection.asme.org/electrochemical/article-pdf/doi/10.1115/1.4042063/6133331/jeecs_016_03_031002.pdf

Reference78 articles.

1. Review of Computational Heat and Mass Transfer Modeling in Polymer-Electrolyte-Membrane (PEM) Fuel Cells;Energy,2008

2. A Review of Polymer Electrolyte Membrane Fuel Cells: Technology, Applications, and Needs on Fundamental Research;Appl. Energy,2011

3. A Critical Review of Modeling Transport Phenomena in Polymer-Electrolyte Fuel Cells;J. Electrochem. Soc.,2014

4. Numerical Analysis of Effects of Gas Crossover Through Membrane Pinholes in High-Temperature Proton Exchange Membrane Fuel Cells;Int. J. Hydrogen Energy,2014

5. Cell Resistances of Poly(2,5-Benzimidazole)-Based High Temperature Polymer Membrane Fuel Cell Membrane Electrode Assemblies: Time Dependence and Influence of Operating Parameters;J. Power Sources,2010

Cited by 8 articles. 订阅此论文施引文献订阅此论文施引文献，注册后可以免费订阅5篇论文的施引文献，订阅后可以查看论文全部施引文献

1. openFuelCell2: A New Computational Tool for Fuel Cells, Electrolyzers, and Other Electrochemical Devices and Processes;Computer Physics Communications;2024-01

2. A new procedure for rapid convergence in numerical performance calculations of electrochemical cells;Electrochimica Acta;2023-12

3. Fuel Cell Types, Properties of Membrane, and Operating Conditions: A Review;Sustainability;2022-11-07

4. High-Efficiency Combined Heat and Power through a High-Temperature Polymer Electrolyte Membrane Fuel Cell and Gas Turbine Hybrid System;Sustainability;2021-11-12

5. A multi‐input and single‐output voltage control for a polymer electrolyte fuel cell system using model predictive control method;International Journal of Energy Research;2021-03-13