Biosynthesis of the Marine Antibiotic Pentabromopseudilin. 2. The Pyrrole Ring

Author:

PESCHKE Jörg D.,HANEFELD Ulf,LAATSCH Hartmut

Publisher

Oxford University Press (OUP)

Subject

Organic Chemistry,Molecular Biology,Applied Microbiology and Biotechnology,General Medicine,Biochemistry,Analytical Chemistry,Biotechnology

Reference2 articles.

1. 17) Obtained from Cambridge Isotope Laboratories, contained: alanine (7.3%), arginine (6.8%), asparatic acid (9.5%), glutamic acid (10.4%), glycine (6.2%), histidine (1.9%), isoleucine (4.0%), leucine (10.6%), lysine (13.7%), methionine (1.0%), phenylalanine (4.5%), proline (6.5%), serine (4.1%), threonine (4.6%), tyrosine (3.9%) and valine (5.1%). 500 mg of this mixture ofL-[U-13C]amino acids was dissolved in 1 liter of the medium.

2. 19) A clear1JC5–C1′=69.5 Hz was visible, but C1′ was not labelled. However, given the high incorporation rate at C5, approximately 30% of13C at C1′ had a13C at C5 as a neighbour. Due to the close proximity of the signals to one another, the1Jand2Jcoupling of C2, C3 and C4 cannot be unambiguously assigned.

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