Simulations of Mixtures of Fluids in Chemical Equilibrium at High Pressures

Author:

Cinnella Pasquale1,Gaiaschi Pietro1

Affiliation:

1. Mississippi State University

Publisher

American Institute of Aeronautics and Astronautics

Reference63 articles.

1. In the following, the generalized EoS for mixtures of fluids is summarized, including details on how to deal with mixtures that are chemically reacting. Then the HBMS single-species EoS is introduced,4-6and a few necessary thermodynamic properties are derived, including fugacities. Numerical results are presented for a simple air dissociation mixture, with the goal of assessing the importance of deviations from the singlespecies thermally perfect laws. Next, a simple combustion mixture is examined involving hydrogen and oxygen, and detailed results are obtained to assess the effects of having most of the non-monoatomic species follow the HBMS EoS.

2. At this point, Eq. (5) can be used as an Equation of State: what one needs is a complete set of pure substance EoS that would yield species specific volumes for a given pressure and temperature. A few simple EoS have been investigated in a previous study.2The more complicated (and accurate) HBMS formula4-6will be investigated in the present study. This EoS is commonly used in combustion problems.

3. k [X]k≡T.

4. A general species EoS that has been widely used in combustion problems is the one originally developed byHirshfelderetal.4-6denotedhereastheHBMSEoS.Itfollowsthegeneralfunctionalformp = pi(T, (v)∗i), which was employed before, however, it features different forms in the gasf, dense gasg, and liquidhregions of the state diagram.

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