Preparation and properties of Y, Mn-doped LMO solid electrolyte for IT-SOFCs

Author:

Yang Jie1ORCID,Dong Li1,Shao Lingbo1,Wei Qing1,Qin Guangchao1,Tian Changan2

Affiliation:

1. School of Energy Materials and Chemical Engineering, Hefei University, Hefei 230601, P. R. China

2. School of Chemistry and Civil Engineering, Shaoguan University, Shaoguan, Guangdong, 512005, P. R. China

Abstract

La2Mo2O9 doped with cheap metal cations can further increase their conductivity. The transition metal element Mn and the rare-earth element Y co-doped La2Mo2O9-based electrolyte was used, and the sintered ceramic body La[Formula: see text]Y[Formula: see text]Mo [Formula: see text][Formula: see text]Mn[Formula: see text]O [Formula: see text][Formula: see text]([Formula: see text]= 0[Formula: see text]0.4) was prepared by the sol-gel method, sintering at 950°C. The results show that the samples can suppress the phase transition and retain the [Formula: see text]-phase of the structure of La2Mo2O9, due to doping, and it is a single pure phase, which has good sintering performance. Among them, La[Formula: see text]Y [Formula: see text]Mo[Formula: see text]Mn[Formula: see text]O[Formula: see text] reached the maximum ionic conductivity of 0.0292 S⋅cm[Formula: see text] at 800°C, and Ea is 0.425 eV, which can become a solid electrolyte material of IT-SOFC.

Funder

excellent young talents fund project in Universities of Anhui Province

Hefei University Quality Engineering Demonstration Experimental Training Center Project

Hefei University Provincial Quality Engineering Demonstration Chemical Experiment Training Center Project

Hefei University Undergraduate Quality Engineering Project

National Natural Science Foundation Project

Anhui Province key research and development program

Anhui Province Natural Science Foundation Project

Guangdong Provincial Ordinary University Characteristic Innovation Project

excellent scientific research and innovation team of colleges and universities in Anhui Province

Publisher

World Scientific Pub Co Pte Ltd

Subject

General Materials Science

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