Enhanced Visible-Light Photocatalytic Remediation of Tetracycline Hydrochloride by Nanostructured BiOI Homojunctions

Author:

Qiao Mengzhu1,Liu Hongjin1,Lv Jun12ORCID,Xu Guangqing12,Zhang Xinyi3,Shu Xia12,Wu Yucheng12

Affiliation:

1. School of Materials Science and Engineering, Hefei University of Technology, Hefei 230009, P. R. China

2. Key Laboratory of Advanced Functional Materials and Devices of Anhui Province, Hefei 230009, P. R. China

3. School of Chemistry, Monash University, Clayton, VIC 3800, Australia

Abstract

The BiOI homojunctions were constructed between BiOI nanosheets and BiOI nanoflowers, which were prepared with a facile ultrasound-assisted solvothermal method. BiOI nanosheets were uniformly distributed on BiOI nanoflowers surface. The homojunction structure constructed between nanosheets and nanoflowers efficiently speeds up the transfer and separation of photoinduced charge carriers, which is beneficial to promote the photocatalytic activity. Compared with single BiOI, BiOI homojunctions exhibit remarkably improved photocatalytic degradation activity for tetracycline hydrochloride (TC); photodegradation rate of 69.43% for TC has been reached after being irradiated under visible light for 1[Formula: see text]h. Deeper analyses of photocatalytic degradation mechanism of TC have been conducted; the results identify that [Formula: see text] and h[Formula: see text] play important roles during the TC degradation reaction.

Funder

the National Natural Science Foundation of China

Natural Science Foundation of Anhui Province

the Fundamental Research Funds for the Central Universities

the 111 Project "New Materials and Technology for Clean Energy"

Publisher

World Scientific Pub Co Pte Lt

Subject

Condensed Matter Physics,General Materials Science

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