Coherent phase control of population transfer through ladder system in two laser pulses with ω and nω

Abstract

The ladder transitions controlled by two harmonic pulses are investigated theoretically using a time-dependent quantum wave packet method for the ground electronic state of HF molecule. By choosing [Formula: see text], [Formula: see text] and [Formula: see text] schemes, the population can be transferred to target states [Formula: see text]. The population distribution can be controlled by the average amplitude of total electric field which depends on the relative phase of two pulses. With the variation of the relative phase between [Formula: see text] and [Formula: see text] pulses, the variation of population has a period of [Formula: see text]. For [Formula: see text] and [Formula: see text] schemes, the population distributions show oscillation behavior with a period of [Formula: see text] by varying the relative phase. The two harmonic pulses can realize a nearly complete population transfer to the target state.