Generation of the high-intensity single harmonic energy peak and attosecond pulse by using resonance ionization schemes from atoms and molecules

Abstract

The lower harmonic intensity is still the reason that limits the application of attosecond pulse. Thus, in this paper, on the basis of resonance ionization schemes, we propose the effective methods to improve the harmonic intensity of atomic and molecular systems. For atomic system (i.e. He atom), with the combination of chirped-UV pulse, not only the harmonic cutoff can be extended, but also the harmonic intensity can be enhanced, caused by the UV resonance ionization between ground state and excited state. As a result, the single harmonic energy peak (HEP) with the higher intensity and higher emitted photon energy can be obtained, which can support the attosecond pulses shorter than 40 as. For the molecular system (i.e. [Formula: see text] and [Formula: see text]), by properly choosing the pulse duration of the fundamental pulse, the time region of charge resonance enhanced ionization (CREI) can be well controlled. Therefore, the maximum HEP with the higher intensity can be obtained. Second, by properly adding a half-cycle unipolar pulse, the selected maximum HEP in the CREI region can be further extended. Thus, an intense and broad spectral region can be produced, which can generate the attosecond pulses with durations of 36[Formula: see text]as.