NONLINEAR OPTICAL PROPERTIES OF AU:TiO2 MULTILAYER COMPOSITE FILMS

Author:

YU S. W.1,LIAO H. B.2,WEN W. J.3,WONG G. K. L.3

Affiliation:

1. Department of Electronic Information Material, School of Materials Science and Engineering, Shanghai University, No. 149, Yanchang Road, Shanghai 200072, China

2. Department of Physics, Beijing Normal University, Beijing 100875, China

3. Department of Physics, the Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong, China

Abstract

Au:TiO 2 multilayer composite films were prepared by the method of alternating multitarget magnetron sputtering technique. Samples were annealed afterwards. The surface plasmon resonances of the annealed films are around 700nm. TEM pictures showed the remained layered structure with grown gold particles between the layers. The values of χ(3) measured by degenerated four wave mixing (DFWM) are in the order of 10-7 esu which are one order larger than the previous work. The figure of merit (FOM), χ(3)/α, is in the order of 10-12 esu cm. The great improvement of χ(3) is assumed to be the result from the enhancement of field localization caused by the metallic/dielectric host multilayer structure.

Publisher

World Scientific Pub Co Pte Lt

Subject

Condensed Matter Physics,Statistical and Nonlinear Physics

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