The use of nanovibration to discover specific and potent bioactive metabolites that stimulate osteogenic differentiation in mesenchymal stem cells

Author:

Hodgkinson Thomas,Tsimbouri P. Monica,Llopis-Hernandez Virginia,Campsie Paul,Scurr David,Childs Peter G,Phillips David,Donnelly Sam,Wells Julia A,Salmeron-Sanchez ManuelORCID,Burgess Karl,Alexander Morgan,Vassalli Massimo,Oreffo Richard O.C.,Reid Stuart,France David J,Dalby Matthew JORCID

Abstract

Bioactive metabolites have wide-ranging biological activities and are a potential source of future research and therapeutic tools. Here, we use nanovibrational stimulation to induce the osteogenic differentiation of MSCs, in the absence of off-target differentiation. We show that this differentiation method, which does not rely on the addition of exogenous growth factors to the culture media, provides an artefact-free approach to identifying bioactive metabolites that specifically and potently induce osteogenesis. We first identify a highly specific metabolite as the endogenous steroid, cholesterol sulphate. Next, a screen of other small molecules with a similar steroid scaffold identified fludrocortisone acetate as being both specific and having highly potent osteogenic-inducing activity. These findings demonstrate that physical priciples can be used to identify bioactive metabolites and then metabolite potency can be optimised by examining structure-function relationship.

Publisher

Cold Spring Harbor Laboratory

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