Lacunarity as a quantitative measure of mixing—a micro-CT analysis-based case study on granular materials

Author:

Vásárhelyi Lívia1ORCID,Sebők Dániel1ORCID,Szenti Imre1,Tóth Ádám1,Lévay Sára23,Vajtai Róbert4ORCID,Kónya Zoltán15,Kukovecz Ákos1

Affiliation:

1. Interdisciplinary Excellence Centre, Department of Applied and Environmental Chemistry, University of Szeged , H-6720, Rerrich Béla tér 1 , Szeged, Hungary

2. University of Lyon, INSA-Lyon, CNRS UMR5259, LaMCoS , 69621 Villeurbanne, France

3. Institute for Solid State Physics and Optics, Wigner Research Centre for Physics , Budapest H-1121, Hungary

4. Department of Materials Science and Nanoengineering, Rice University , Houston, TX MS 325, USA

5. ELKH-SZTE Reaction Kinetics and Surface Chemistry Research Group , H-6720 Szeged Rerrich Béla tér 1, Hungary

Abstract

Abstract In practically every industry, mixing is a fundamental process, yet its 3D analysis is scarce in the literature. High-resolution computed tomography (micro-CT) is the perfect X-ray imaging tool to investigate the mixing of granular materials. Other than qualitative analysis, 3D micro-CT images provide an opportunity for quantitative analysis, which is of utmost importance, in terms of efficiency (time and budget) and environmental impact of the mixing process. In this work, lacunarity is proposed as a measure of mixing. By the lacunarity calculation on the repeated micro-CT measurements, a temporal description of the mixing can be given in three dimensions. As opposed to traditional mixing indices, the lacunarity curve provides additional information regarding the spatial distribution of the grains. Discrete element method simulations were also performed and showed similar results to the experiments.

Funder

Ministry of Innovation and Technology of Hungary from the National Research, Development and Innovation Fund

Publisher

Oxford University Press (OUP)

Subject

General Materials Science

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