Human activities aggravate nitrogen-deposition pollution to inland water over China

Author:

Gao Yang12,Zhou Feng3ORCID,Ciais Philippe34,Miao Chiyuan5,Yang Tao6,Jia Yanlong1,Zhou Xudong6,Klaus Butterbach-Bahl7,Yang Tiantian8,Yu Guirui1

Affiliation:

1. Key Laboratory of Ecosystem Network Observation and Modeling, Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing 100101, China

2. State Key Laboratory of Lake Science and Environment, Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing 210008, China

3. Sino-French Institute for Earth System Science, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China

4. Laboratoire des Sciences du Climat et de l’Environnement, CEA CNRS UVSQ, Gif-sur-Yvette 91191, France

5. State Key Laboratory of Earth Surface Processes and Resource Ecology, Beijing Normal University, Beijing 100875, China

6. State Key Laboratory of Hydrology-Water Resources and Hydraulic Engineering, Center for Global Change and Water Cycle, Hohai University, Nanjing 210098, China

7. Institute for Meteorology and Climate Research, Atmospheric Environmental Research, Karlsruhe Institute of Technology, 82467 Garmisch-Partenkirchen, Germany

8. Department of Civil and Environmental Engineering, University of California, Irvine, CA 92697, USA

Abstract

Abstract In the past three decades, China has built more than 87 000 dams with a storage capacity of ≈6560 km3 and the total surface area of inland water has increased by 6672 km2. Leaching of N from fertilized soils to rivers is the main source of N pollution in China, but the exposure of a growing inland water area to direct atmospheric N deposition and N leaching caused by N deposition on the terrestrial ecosystem, together with increased N deposition and decreased N flow, also tends to raise N concentrations in most inland waters. The contribution of this previously ignored source of  N deposition to freshwaters is estimated in this study, as well as mitigation strategies. The results show that the annual amounts of N depositions ranged from 4.9 to 16.6 kg · ha−1 · yr−1 in the 1990s to exceeding 20 kg · ha−1 · yr−1 in the 2010s over most of regions in China, so the total mass of ΔN (the net contribution of N deposition to the increase in N concentration) for lakes, rivers and reservoirs change from 122.26 Gg N · yr−1 in the 1990s to 237.75 Gg N · yr−1 in the 2010s. It is suggested that reducing the N deposition from various sources, shortening the water-retention time in dams and decreasing the degree of regulation for rivers are three main measures for preventing a continuous increase in the N-deposition pollution to inland water in China.

Funder

National Natural Science Foundation of China

National Key R&D Program of China

Youth Innovation Promotion Association

Chinese Academy of Sciences

Publisher

Oxford University Press (OUP)

Subject

Multidisciplinary

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