A dynamically stable self-healable wire based on mechanical–electrical coupling

Author:

Wang Shuo1,Ouyang Zhaofeng1,Geng Shitao1,Wang Yan1,Zhao Xiaoju1,Yuan Bin1,Zhang Xiao1,Xu Qiuchen1,Tang Chengqiang2,Tang Shanshan1,Miao Han3,Peng Huisheng2,Sun Hao1ORCID

Affiliation:

1. Frontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Zhangjiang Institute for Advanced Study, and Key Laboratory of Green and High-End Utilization of Salt Lake Resources (Chinese Academy of Sciences), Shanghai Jiao Tong University , Shanghai 200240 , China

2. State Key Laboratory of Molecular Engineering of Polymers, Department of Macromolecular Science, Institute of Fiber Materials and Devices, and Laboratory of Advanced Materials, Fudan University , Shanghai 200438 , China

3. School of Materials Science and Engineering, East China University of Science and Technology , Shanghai 200433 , China

Abstract

ABSTRACT The rise in wearable electronics has witnessed the advancement of self-healable wires, which are capable of recovering mechanical and electrical properties upon structural damage. However, their highly fluctuating electrical resistances in the range of hundreds to thousands of ohms under dynamic conditions such as bending, pressing, stretching and tremoring may seriously degrade the precision and continuity of the resulting electronic devices, thus severely hindering their wearable applications. Here, we report a new family of self-healable wires with high strengths and stable electrical conductivities under dynamic conditions, inspired by mechanical–electrical coupling of the myelinated axon in nature. Our self-healable wire based on mechanical–electrical coupling between the structural and conductive components has significantly improved the electrical stability under dynamic scenarios, enabling precise monitoring of human health status and daily activities, even in the case of limb tremors from simulated Parkinson's disease. Our mechanical–electrical coupling strategy opens a new avenue for the development of dynamically stable electrodes and devices toward real-world wearable applications.

Funder

National Natural Science Foundation of China

Fundamental Research Funds for the Central Universities

Shanghai Pujiang Program

Publisher

Oxford University Press (OUP)

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