Investigating the frequency and trends in global above-cloud aerosol characteristics with CALIOP and OMI

Abstract

Abstract. Seven and a half years (June 2006–November 2013) of Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) aerosol and cloud layer products are compared with collocated Ozone Monitoring Instrument (OMI) Aerosol Index (AI) data and Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) cloud products, to investigate variability in estimates of bi-annual and monthly above-cloud aerosol (ACA) events globally. The active- (CALIOP) and passive-based (OMI-MODIS) techniques have their advantages and caveats for ACA detection, and thus both are used to get a thorough and robust comparison of daytime cloudy-sky ACA distribution and climatology. For the first time, baseline above-cloud aerosol optical depth (ACAOD) and AI thresholds are derived and examined (AI = 1.0, ACAOD = 0.015) for each sensor. Both OMI-MODIS and CALIOP-based daytime spatial distributions of ACA events show similar patterns during both study periods (December–May) and (June–November). Divergence exists in some regions, however, such as Southeast Asia during June through November, where daytime cloudy-sky ACA frequencies of up to 10% are found from CALIOP yet are non-existent from the OMI-based method. Conversely, annual cloudy-sky ACA frequencies of 20–30% are reported over Northern Africa from the OMI-based method, yet are largely undetected by the CALIOP-based method. This is possibly due to a misclassification of thick dust plumes as clouds by the OMI-MODIS based method. An increasing trend of ~0.5% per year (since 2009) in global monthly cloudy-sky ACA daytime frequency of occurrence is found using the OMI-MODIS based method. Yet, CALIOP-based global daytime ACA frequencies exhibit a near-zero trend. Further analysis suggests that the OMI derived cloudy-sky ACA frequency trend may be affected by OMI row anomalies in later years. A few regions are found to have increasing trends of cloudy-sky ACA frequency, including the Middle-East and India. Regions with slightly negative cloudy-sky ACA frequency trends are found over South America and the Southern Oceans, while remaining regions in the study show a near-zero trend. Global and regional trends are not statistically significant, though, given relatively lacking sample sizes. A longer data record of ACA events is needed in order to establish a more significant trend of ACA frequency regionally and globally.