Black carbon aerosol reductions during COVID-19 confinement quantified by aircraft measurements over Europe
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Published:2022-07-06
Issue:13
Volume:22
Page:8683-8699
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ISSN:1680-7324
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Container-title:Atmospheric Chemistry and Physics
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language:en
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Short-container-title:Atmos. Chem. Phys.
Author:
Krüger Ovid O.ORCID, Holanda Bruna A., Chowdhury SourangsuORCID, Pozzer AndreaORCID, Walter DavidORCID, Pöhlker ChristopherORCID, Andrés Hernández Maria Dolores, Burrows John P.ORCID, Voigt ChristianeORCID, Lelieveld JosORCID, Quaas JohannesORCID, Pöschl UlrichORCID, Pöhlker Mira L.
Abstract
Abstract. The abrupt reduction in human activities during the first lockdown of the COVID-19 pandemic created unprecedented atmospheric conditions. To quantify the changes in lower tropospheric air pollution, we conducted the BLUESKY aircraft campaign and measured vertical profiles of black carbon (BC) aerosol particles over western and southern Europe in May and June 2020. We compared the results to similar measurements of the EMeRGe EU campaign performed in July 2017 and found that the BC mass concentrations (MBC) were reduced by about 48 %. For BC particle number concentrations, we found comparable reductions. Based on ECHAM/MESSy Atmospheric Chemistry (EMAC) chemistry-transport model simulations, we found differences in meteorological conditions and flight patterns responsible for about 7 % of the MBC reductions. Accordingly 41 % of MBC reductions can be attributed to reduced anthropogenic emissions. Our results reflect the strong and immediate positive effect of changes in human activities on air quality and the atmospheric role of BC aerosols as a major air pollutant in the Anthropocene.
Funder
Deutsche Forschungsgemeinschaft
Publisher
Copernicus GmbH
Subject
Atmospheric Science
Reference84 articles.
1. Andreae, M. O.: Aerosols Before Pollution, Science, 315, 50–51,
https://doi.org/10.1126/science.1136529, 2007. a 2. Andreae, M. O., Afchine, A., Albrecht, R., Holanda, B. A., Artaxo, P., Barbosa, H. M. J., Borrmann, S., Cecchini, M. A., Costa, A., Dollner, M., Fütterer, D., Järvinen, E., Jurkat, T., Klimach, T., Konemann, T., Knote, C., Krämer, M., Krisna, T., Machado, L. A. T., Mertes, S., Minikin, A., Pöhlker, C., Pöhlker, M. L., Pöschl, U., Rosenfeld, D., Sauer, D., Schlager, H., Schnaiter, M., Schneider, J., Schulz, C., Spanu, A., Sperling, V. B., Voigt, C., Walser, A., Wang, J., Weinzierl, B., Wendisch, M., and Ziereis, H.: Aerosol characteristics and particle production in the upper troposphere over the Amazon Basin, Atmos. Chem. Phys., 18, 921–961, https://doi.org/10.5194/acp-18-921-2018, 2018. a, b 3. Andrés Hernández, M. D., Hilboll, A., Ziereis, H., Förster, E., Krüger, O. O., Kaiser, K., Schneider, J., Barnaba, F., Vrekoussis, M., Schmidt, J., Huntrieser, H., Blechschmidt, A.-M., George, M., Nenakhov, V., Harlass, T., Holanda, B. A., Wolf, J., Eirenschmalz, L., Krebsbach, M., Pöhlker, M. L., Kalisz Hedegaard, A. B., Mei, L., Pfeilsticker, K., Liu, Y., Koppmann, R., Schlager, H., Bohn, B., Schumann, U., Richter, A., Schreiner, B., Sauer, D., Baumann, R., Mertens, M., Jöckel, P., Kilian, M., Stratmann, G., Pöhlker, C., Campanelli, M., Pandolfi, M., Sicard, M., Gómez-Amo, J. L., Pujadas, M., Bigge, K., Kluge, F., Schwarz, A., Daskalakis, N., Walter, D., Zahn, A., Pöschl, U., Bönisch, H., Borrmann, S., Platt, U., and Burrows, J. P.: Overview: On the transport and transformation of pollutants in the outflow of major population centres – observational data from the EMeRGe European intensive operational period in summer 2017, Atmos. Chem. Phys., 22, 5877–5924, https://doi.org/10.5194/acp-22-5877-2022, 2022. a, b, c 4. Ban-Weiss, G. A., McLaughlin, J. P., Harley, R. A., Lunden, M. M.,
Kirchstetter, T. W., Kean, A. J., Strawa, A. W., Stevenson, E. D., and
Kendall, G. R.: Long-term changes in emissions of nitrogen oxides and
particulate matter from on-road gasoline and diesel vehicles, Atmos.
Environ., 42, 220–232, https://doi.org/10.1016/j.atmosenv.2007.09.049, 2008. a 5. Ban-Weiss, G. A., Lunden, M. M., Kirchstetter, T. W., and Harley, R. A.:
Measurement of black carbon and particle number emission factors from
individual heavy-duty trucks, Environ. Sci. Technol., 43,
1419–1424, https://doi.org/10.1021/es8021039, 2009. a
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