UK surface NO<sub>2</sub> levels dropped by 42 % during the COVID-19 lockdown: impact on surface O<sub>3</sub>
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Published:2020-12-18
Issue:24
Volume:20
Page:15743-15759
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ISSN:1680-7324
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Container-title:Atmospheric Chemistry and Physics
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language:en
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Short-container-title:Atmos. Chem. Phys.
Author:
Lee James D.ORCID, Drysdale Will S.ORCID, Finch Doug P.ORCID, Wilde Shona E.ORCID, Palmer Paul I.ORCID
Abstract
Abstract. We report changes in surface nitrogen dioxide (NO2) across the UK during the COVID-19
pandemic when large and rapid emission reductions accompanied a nationwide lockdown (23 March–31
May 2020, inclusively), and compare them with values from an equivalent period over the previous
5 years. Data are from the Automatic Urban and Rural Network (AURN), which forms the basis of
checking nationwide compliance with ambient air quality directives. We calculate that
NO2 reduced by 42 %±9.8 % on average across all 126 urban AURN sites, with a
slightly larger (48 %±9.5 %) reduction at sites close to the roadside (urban traffic). We
also find that ozone (O3) increased by 11 % on average across the urban background
network during the lockdown period. Total oxidant levels
(Ox=NO2+O3) increased only slightly on average
(3.2 %±0.2 %), suggesting the majority of this change can be attributed to photochemical
repartitioning due to the reduction in NOx. Generally, we find larger, positive
Ox changes in southern UK cities, which we attribute to increased UV radiation
and temperature in 2020 compared to previous years. The net effect of the NO2 and
O3 changes is a sharp decrease in exceedances of the NO2 air quality objective
limit for the UK, with only one exceedance in London in 2020 up until the end of May. Concurrent
increases in O3 exceedances in London emphasize the potential for O3 to become
an air pollutant of concern as NOx emissions are reduced in the next
10–20 years.
Funder
Natural Environment Research Council
Publisher
Copernicus GmbH
Subject
Atmospheric Science
Reference46 articles.
1. An, Z., Jin, Y., Li, J., Li, W., and Wu, W.: Impact of Particulate Air Pollution on
Cardiovascular Health, Current Allergy and Asthma Reports, 18, 15,
https://doi.org/10.1007/s11882-018-0768-8, 2018. 2. Bao, R., and Zhang, A.: Does lockdown reduce air pollution? Evidence from 44 cities in
northern China, Sci. Total Environ., 731, 139052, https://doi.org/10.1016/j.scitotenv.2020.139052, 2020. 3. Bekbulat, B., Apte, J., Millet, D., Robinson, A., Wells, K., and Marshall, J.:
PM2.5 and Ozone Air Pollution Levels Have Not Dropped Consistently Across the US
Following Societal Covid Response, 2020. 4. Cooper, O. R., Gao, R.-S., Tarasick, D., Leblanc, T., and Sweeney, C.: Long-term ozone
trends at rural ozone monitoring sites across the United States, 1990–2010. J. Geophys. Res.,
117, D22307, https://doi.org/10.1029/2012JD018261, 2012. 5. Cooper, O. R., Parrish, D. D, Ziemke, J., Balashov, N. V., Cupeiro, M., Galbally,
I. E., Gilge, Horowitz, S., Jensen, L. H., Lamarque, J.-F., Naik, V., Oltmans, S., Schwab, J.,
Shindell, D. T., Thompson, A. M., Thouret, V., Wang, Y., and Zbinden, R. M.: Global distribution and
trends of tropospheric ozone: An observation-based review, Elem. Sci. Anth., 2, 29, https://doi.org/10.12952/journal.elementa.000029, 2014.
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