Big grains go far: reconciling tephrochronology with atmospheric measurements of volcanic ash

Abstract

Abstract. There is a large discrepancy between the size of volcanic ash particles measured from deposits on the ground (known as cryptotephra; 20–125 μm in length) and those reported by satellite remote sensing (effective radii of 0.5–9 μm; 95% of particles < 17 μm diameter). We use results from the fields of tephrochronology (a dating technique based on volcanic ash layers), dispersion modelling and satellite remote sensing in an attempt to understand from where it arises. We show that Icelandic cryptotephras deposited in NW Europe have lognormal particle size distributions (PSDs) with median lengths of 20–70 μm (geometric standard deviation: 1.40–1.66; 95th percentile length: 42–126 microns). This is consistent with semi-quantitative grainsize range estimates from the literature. Using measured fall velocities of ash particles, a release height typical of moderate Icelandic eruptions (10 km) and a wind speed typical for NW Europe (10 m s−1), we find that an ash cloud can transport particles < 80 μm diameter up to 850 km in 24 h, so that even moderately sized Icelandic eruptions can deposit cryptotephra on mainland Europe. The proportion of cryptotephra in airborne clouds is unknown. We used simulated satellite data of dispersion-model-derived ash clouds to investigate the effect of PSD on satellite retrievals and show that as the median radius of the input PSD increases, fewer ash-containing pixels are correctly identified. Where retrievals are made of simulated clouds with mass median radii larger than ~ 10 μm, the mean retrieved reff plateaus at around 9 μm. This is a systematic bias in the retrieval algorithm that would cause the grainsize of distal clouds containing significant cryptotephra to be underestimated. This cannot explain discrepancies in coarser proximal clouds, however, which may be because the complex physics of scattering by highly irregularly-shaped grains is inadequately represented by assuming that particles are dense spheres.