Transported aerosols regulate the pre-monsoon rainfall over north-east India: a WRF-Chem modelling study
-
Published:2023-06-07
Issue:11
Volume:23
Page:6197-6215
-
ISSN:1680-7324
-
Container-title:Atmospheric Chemistry and Physics
-
language:en
-
Short-container-title:Atmos. Chem. Phys.
Author:
Barman NeeldipORCID, Gokhale Sharad
Abstract
Abstract. The study differentiates and quantifies the impacts of aerosols
emitted locally within the north-east (NE) India region and those transported
from outside this region to ascertain whether local or transported aerosols
are more impactful in influencing this region's rainfall during the
pre-monsoon season (March–April–May). Due to the existence of a declining
pre-monsoon rainfall trend in NE India, the study also quantified the role
of different aerosol effects in radiative forcing (RF) and rainfall. The
study has been carried out using the WRF-Chem model by comparing simulation
scenarios where emissions were turned on and off within and outside the NE
region. The impact of all emissions as a whole and black carbon (BC)
specifically was studied. Results show that aerosols transported primarily
from the Indo-Gangetic Plain (IGP) were responsible for 93.98 % of the
PM10 mass over NE India's atmosphere and 64.18 % of near-surface
PM10 concentration. Transported aerosols contributed >50 % of BC, organic carbon, sulfate, nitrate, ammonium and dust aerosol
concentration and are hence a major contributor to air pollution. Hence, the
aerosol effects were much greater with transported aerosols. An indirect
aerosol effect was found to be the major effect and more impactful, with
transported aerosols that dominated both rainfall and RF and suppressed
rainfall more significantly than the direct and semi-direct effect. However, the
increase in direct radiative effects with an increase in transported BC
counteracted the rainfall suppression caused by relevant processes of other
aerosol effects. Thus, this study shows atmospheric transport to be an
important process for this region, as transported emissions, specifically
from the IGP, were also found to have greater control over the region's rainfall.
Thus, emission control policies implemented in the IGP will reduce air pollution
as well as the climatic impacts of aerosols over the NE India region.
Publisher
Copernicus GmbH
Subject
Atmospheric Science
Reference85 articles.
1. Bagtasa, G., Cayetano, M. G., Yuan, C. S., Uchino, O., Sakai, T., Izumi, T.,
Morino, I., Nagai, T., Macatangay, R. C., and Velazco, V. A.: Long-range
transport of aerosols from East and Southeast Asia to northern Philippines
and its direct radiative forcing effect, Atmos. Environ., 218, 117007,
https://doi.org/10.1016/j.atmosenv.2019.117007, 2019. 2. Barman, N. and Gokhale, S.: Urban black carbon - source apportionment,
emissions and long-range transport over the Brahmaputra River Valley, Sci.
Total Environ., 693, 1–14, https://doi.org/10.1016/j.scitotenv.2019.07.383,
2019. 3. Barman, N. and Gokhale, S.: Aerosol influence on the pre-monsoon rainfall
mechanisms over North-East India: A WRF-Chem study, Atmos. Res., 268,
106002, https://doi.org/10.1016/j.atmosres.2021.106002, 2022. 4. Bauer, S. E. and Menon, S.: Aerosol direct, indirect, semidirect, and surface albedo effects from sector contributions based on the IPCC AR5 emissions for preindustrial and present-day conditions, J. Geophys. Res.-Atmos., 117, https://doi.org/10.1029/2011JD016816, 2012. 5. Bhat, M. A., Romshoo, S. A., and Beig, G.: Characteristics, source
apportionment and long-range transport of black carbon at a high-altitude
urban centre in the Kashmir valley, North-western Himalaya, Environ.
Pollut., 305, 119295, https://doi.org/10.1016/j.envpol.2022.119295, 2022.
|
|