Abstract
Abstract. Low-cost air quality sensors offer significant potential for
enhancing urban air quality networks by providing higher-spatiotemporal-resolution data needed, for example, for evaluation of air quality
interventions. However, these sensors present methodological and deployment
challenges which have historically limited operational ability. These
include variability in performance characteristics and sensitivity to
environmental conditions. In this work, we investigate field “baselining”
and interference correction using random forest regression methods for
low-cost sensing of NO2, PM10 (particulate matter) and PM2.5. Model performance
is explored using data obtained over a 7-month period by real-world field
sensor deployment alongside reference method instrumentation. Workflows and
processes developed are shown to be effective in normalising variable sensor
baseline offsets and reducing uncertainty in sensor response arising from
environmental interferences. We demonstrate improvements of between 37 %
and 94 % in the mean absolute error term of fully corrected sensor
datasets; this is equivalent to performance within ±2.6 ppb of the reference
method for NO2, ±4.4 µg m−3 for PM10 and ±2.7 µg m−3 for PM2.5. Expanded-uncertainty estimates for PM10
and PM2.5 correction models are shown to meet performance criteria
recommended by European air quality legislation, whilst that of the NO2
correction model was found to be narrowly (∼5 %) outside of
its acceptance envelope. Expanded-uncertainty estimates for corrected sensor
datasets not used in model training were 29 %, 21 % and 27 % for
NO2, PM10 and PM2.5 respectively.
Funder
National Institute for Health Research
Natural Environment Research Council
Reference42 articles.
1. Alphasense Ltd.: NO2-A43F Nitrogen Dioxide Sensor 4-Electrode Technical
Specification, https://www.alphasense.com/wp-content/uploads/2019/09/NO2-A43F.pdf (last access: 19 May 2021), 2019a.
2. Alphasense Ltd.: OPC-N3 Particle Monitor Technical Specification,
https://www.alphasense.com/wp-content/uploads/2019/03/OPC-N3.pdf (last access: 19 May 2021), 2019b.
3. Berrar, D.: Cross-validation, in Encyclopaedia of Bioinformatics and
Computational Biology: ABC of Bioinformatics, Elsevier, 3, 542–545,
2018.
4. Bigi, A., Mueller, M., Grange, S. K., Ghermandi, G., and Hueglin, C.: Performance of NO, NO2 low cost sensors and three calibration approaches within a real world application, Atmos. Meas. Tech., 11, 3717–3735, https://doi.org/10.5194/amt-11-3717-2018, 2018.
5. Breiman, L.: Bagging predictors, Mach. Learn., 24, 123–140,
https://doi.org/10.1023/A:1018054314350, 1996.
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