Influence of cloud processing on CCN activation behaviour in the Thuringian Forest, Germany during HCCT-2010
Author:
Henning S., Dieckmann K., Ignatius K., Schäfer M.ORCID, Zedler P., Harris E.ORCID, Sinha B.ORCID, van Pinxteren D., Mertes S., Birmili W., Merkel M., Wu Z., Wiedensohler A., Wex H.ORCID, Herrmann H.ORCID, Stratmann F.
Abstract
Abstract. Within the framework of the international cloud experiment "Hill Cap Cloud Thuringia 2010" (HCCT-2010), the influence of cloud processing on the activation properties of ambient aerosol particles was investigated. Particles were probed up- and downwind of an orographic cap cloud on Mt. Schmücke, which is part of a large mountain ridge in Thuringia, Germany. The activation properties of the particles were investigated by means of size-segregated Cloud Condensation Nuclei (CCN) measurements at 3 to 4 different supersaturations. The observed CCN spectra together with the total particle spectra were used to calculate the hygroscopicity parameter κ for the up- and the downwind stations. The up- and downwind critical diameters and κ values were then compared for defined Cloud Events and Non Cloud Events. Cloud processing was found to significantly increase the hygroscopicity of the aerosol particles, with an average increase in κ of 50%. Mass spectrometry analysis and isotopic analysis of the particles show that the observed increase in hygroscopicity of the cloud-processed particles is due to an enrichment of nitrate and sulfate in the particle phase.
Publisher
Copernicus GmbH
Reference37 articles.
1. Birmili, W., Stratmann, F., and Wiedensohler, A.: Design of a DMA-based size spectrometer for a large particle size range and stable operation, J. Aerosol Sci., 30, 549–553, 1999. 2. Bower, B. K. N., Choularton, T. W., Gallagher, M. W., Beswick, K. M., Flynn, M. J., Allen, A. G., Davison, B. M., James, J. D., Robertson, L., Harrison, R. M., Hewitt, C. N., Cape, J. N., McFadyen, G. G., Milford, C., Sutton, M. A., Martinsson, B. G., Frank, G., Swietlicki, E., Zhou, J., Berg, O. H., Mentes, B., Papaspiropoulos, G., Hansson, H. C., Leck, C., Kulmala, M., Aalto, P., Vakeva, M., Berner, A., Bizjak, M., Fuzzi, S., Laj, P., Facchini, M. C., Orsi, G., Ricci, L., Nielsen, M., Allan, B. J., Coe, H., McFiggans, G., Plane, J. M. C., Collett, J. L., Moore, K. F., and Sherman, D. E.: ACE-2 HILLCLOUD: an overview of the ACE-2 ground-based cloud experiment, Tellus B, 52, 750–778, 2000. 3. Bower, K. N., Choularton, T. W., Gallagher, M. W., Colvile, R. N., Beswick, K. M., Inglis, D. W. F., Bradbury, C., Martinsson, B. G., Swietlicki, E., Berg, O. H., Cederfelt, S. I., Frank, G., Zhou, J., Cape, J. N., Sutton, M. A., McFadyen, G. G., Milford, C., Birmili, W., Yuskiewicz, B. A., Wiedensohler, A., Stratmann, F., Wendisch, M., Berner, A., Ctyroky, P., Galambos, Z., Mesfin, S. H., Dusek, U., Dore, C. J., Lee, D. S., Pepler, S. A., Bizjak, M., and Divjak, B.: The Great Dun Fell experiment 1995: an overview, Atmos. Res., 50, 151–184, 1999. 4. Choularton, T. W., Colvile, R. N., Bower, K. N., Gallagher, M. W., Wells, M., Beswick, K. M., Arends, B. G., Mols, J. J., Kos, G. P. A., Fuzzi, S., Lind, J. A., Orsi, G., Facchini, M. C., Laj, P., Gieray, R., Wieser, P., Engelhardt, T., Berner, A., Kruisz, C., Moller, D., Acker, K., Wieprecht, W., Luttke, J., Levsen, K., Bizjak, M., Hansson, H. C., Cederfelt, S. I., Frank, G., Mentes, B., Martinsson, B., Orsini, D., Svenningsson, B., Swietlicki, E., Wiedensohler, A., Noone, K. J., Pahl, S., Winkler, P., Seyffer, E., Helas, G., Jaeschke, W., Georgii, H. W., Wobrock, W., Preiss, M., Maser, R., Schell, D., Dollard, G., Jones, B., Davies, T., Sedlak, D. L., David, M. M., Wendisch, M., Cape, J. N., Hargreaves, K. J., Sutton, M. A., StoretonWest, R. L., Fowler, D., Hallberg, A., Harrison, R. M., and Peak, J. D.: The Great Dun Fell cloud experiment 1993: an overview, Atmos. Environ., 31, 2393–2405, https://doi.org/10.1016/s1352-2310(96)00316-0, 1997. 5. DeCarlo, P. F., Kimmel, J. R., Trimborn, A., Northway, M. J., Jayne, J. T., Aiken, A. C., Gonin, M., Fuhrer, K., Horvath, T., Docherty, K. S., Worsnop, D. R., and Jimenez, J. L.: Field-deployable, high-resolution, time-of-flight aerosol mass spectrometer, Anal. Chem., 78, 8281–8289, https://doi.org/10.1021/ac061249n, 2006.
Cited by
3 articles.
订阅此论文施引文献
订阅此论文施引文献，注册后可以免费订阅5篇论文的施引文献，订阅后可以查看论文全部施引文献
|
|