Experimental validation of a CeBr3 gamma-ray logging probe MCNP model

Abstract

Orano Mining has relied on Nuclear Measurement Laboratories for several years to estimate calibration factors for borehole radiometric probes. The total gamma count rate recorded with a NaI(Tl) scintillation detector (NGRS probe) is converted into equivalent uranium grade using a calibration coefficient in s-1.ppmU-1 units, estimated thanks to different calibration blocks ranging from 0 to 10,000 ppm of uranium, at Orano CIME calibration facility in Bessines, France. Recently, Orano Mining embarked on an update of its measurement means by associating gamma spectrometry directly in the wellbore. Therefore, Orano Mining has recently tested a CeBr3 probe designed and developed by ALT (Advanced Logic Technology) to qualify a patented borehole spectroscopic method based on energy bands recently developed by CEA and Orano. In this context, we have implemented a fine Monte Carlo modelling of this new probe in order to correct the calibration coefficients as a function of different parameters such as the drilling diameter, the presence of a casing, the density of the mineralization, the distance of the probe with respect to the well or casing walls, etc. In the present work, we have simulated the CeBr3 probe in the concrete calibration blocks of Orano CIME. The MCNP model of the probe has been validated through a comparison with experimental data. The calibration coefficient determined by simulation is 11.6 s-1.ppm -1 > 10 % in total gamma counting, which is in good agreement with the one measured in Bessines, i.e. 10.6 s-1.ppm -1. The calculation vs. experiment agreement is also satisfactory (i.e. within 10 %) for spectroscopic energy bands used to characterize the uranium grade in case of disequilibrium in the uranium chain, when total count rate does not apply. This method recently developed for samples and boreholes will be tested in future work with this new CeBr3 probe.