Formation of M5Si3 Type Si-Ti-Zr System Intermetallic Compounds by Pulse Electric Current Sintering with Self-Propagating High Temperature Synthesis

Author:

Ikarashi Yukinori1,Nanko Makoto2,Ishizaki Kozo2

Affiliation:

1. Tsuruoka National College of Technology

2. Nagaoka University of Technology

Abstract

Pulse electric current sintering (PECS) is applied to synthesis M5Si3 type Si-Ti-Zr system intermetallic compounds, Si3TixZr(5-x) x=0-5, directly from raw powders of silicon, titanium and zirconium. Almost full conversion to Si3TixZr(5-x) are achieved by PECS method with self-propagating high temperature synthesis (SHS) reaction. The adiabatic temperatures are susceptible to sintering behaviors such as vacuum pressure in chamber and displacement of pressure axis on the PECS process. The large quantities of gases are released in Zr-rich samples. The bulk shapes with almost dense samples are obtained at Ti-rich samples.

Publisher

Trans Tech Publications, Ltd.

Subject

Mechanical Engineering,Mechanics of Materials,General Materials Science

Reference5 articles.

1. P. B. Celis, E. Kagawa and K. Ishizaki, Design and production of the Zr3Ti2Si3 intermetallic compound, J. Mater. Res. 6 (1991) 2077-(2083).

2. P. B. Celis, K. Ishizaki, E. Kagawa and J. Ishikawa, Next generation of high temperature structural intermetallic compounds, Mat. Res. Soc. Symp. Proc. 252 (1992) 9-14.

3. Y. Ikarashi and K. Ishizaki, Forming study on reactive sintering of Si3Zr5 by pulse electric current sintering, ATM 1 (1998) 79-89.

4. A. G. Merzhanov, Fizk. Khim. Soverem. Ploblem. (1983) 7.

5. J. Subrahmanyam and M. Vijayakumar, Self-propagating high-temperature synthesis, J. Mater. Sci. 27 (1992) 6249-6273.

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