Numerical Analysis of Diffusion-Controlled Internal Corrosion by the Cellular Automata Approach

Author:

Krupp Ulrich1,Jahns Katrin1,Balinski Kamil1,Wübbelmann Jürgen1

Affiliation:

1. University of Applied Sciences Osnabrück

Abstract

The cellular automata method offers a promising approach to describe diffusion and diffusion-controlled precipitation processes at high temperatures. During high temperature exposure, technical components like gas-turbine blades, furnaces, or exhaust systems, are operating in corrosive atmospheres. The resulting material-degradation processes are diffusion‐controlled, and corrosive species penetrate into the material leading to the formation of embrittling precipitates. Cellular automata (CA) represent distributed dynamical systems whose structure is particularly well suited to determine the temporal evolution of the system. In this study, it is shown that the model is able to consider diffusion, nucleation and growth aspects, interdiffusion between scales, and high diffusivity paths like grain boundaries. This has been demonstrated by applying CA to (i) nitrogen diffusion, (ii) internal intergranular oxidation of nickel-based alloy, and (iii) interdiffusion of a binary diffusion couple.

Publisher

Trans Tech Publications, Ltd.

Subject

Condensed Matter Physics,General Materials Science,Radiation

Reference28 articles.

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2. L.S. Darken. Diffusion, Mobility and their Interrelation through Free Energy in BinaryMetallic Systems. Transactions of the Metallurgical Society of AIME, 175(1): 184–201, (1948).

3. C. Wagner, Zeitschrift für Elektrochemie 63, 1959 (772).

4. K. Bongartz, R. Schulten, W. J. Quadakkers, H. Nickel, A Finite Difference Model describing Carburization in High-Temperature Alloys, Corrosion 42 (1986), 390.

5. H. G. Sockel, H. ‐J. Christ, Penetration of Foreign Elements Connected with Internal Precipitation: A Computer-Based Description and First Experimental Verification, Materials Science and Engineering 87 (1987), 119.

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