Printable Two-Dimensional V2O5/MXene Heterostructure Cathode for Lithium-Ion Battery

Author:

Wang YangORCID,Lubbers Ties,Xia Rui,Zhang Yi-Zhou,Mehrali Mohammad,Huijben Mark,ten Elshof Johan E.ORCID

Abstract

Two-dimensional nanosheets show promise as electrode materials for high electrochemical performance lithium-ion batteries owing to their unique properties. However, individual nanosheets cannot meet all the required properties for batteries in one material to achieve optimal performance. Here, we demonstrate a new type of two-dimensional heterostructure cathode material for lithium-ion batteries by inkjet printing a composite ink based on high capacity V2O5 nanosheets and high electronic conductivity Ti3C2Tx nanosheets. The excellent electronic conductivity of Ti3C2Tx nanosheets and layer-by-layer heterostructure design enable fast electron transport and minimization of detrimental volume changes during the electrochemical process, respectively. The printed cathodes exhibit a high capacity of 321 mAh g−1 at 1C, high-rate capability of 112 mAh g−1 at 10.5C and good cycling stability after 680 cycles with 91.8% capacity retention, indicating high electrochemical performance of the printed heterostructure cathode. This work opens new opportunities of two-dimensional heterostructures for high performance energy storage applications.

Funder

China Scholarships Council

Publisher

The Electrochemical Society

Subject

Materials Chemistry,Electrochemistry,Surfaces, Coatings and Films,Condensed Matter Physics,Renewable Energy, Sustainability and the Environment,Electronic, Optical and Magnetic Materials

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