Cleaner Skies during the COVID-19 Lockdown

Author:

Voigt Christiane1,Lelieveld Jos2,Schlager Hans3,Schneider Johannes2,Curtius Joachim4,Meerkötter Ralf3,Sauer Daniel3,Bugliaro Luca3,Bohn Birger5,Crowley John N.2,Erbertseder Thilo3,Groß Silke3,Hahn Valerian1,Li Qiang3,Mertens Mariano3,Pöhlker Mira L.6,Pozzer Andrea2,Schumann Ulrich3,Tomsche Laura1,Williams Jonathan2,Zahn Andreas7,Andreae Meinrat8,Borrmann Stephan9,Bräuer Tiziana3,Dörich Raphael2,Dörnbrack Andreas3,Edtbauer Achim2,Ernle Lisa2,Fischer Horst2,Giez Andreas3,Granzin Manuel4,Grewe Volker10,Harder Hartwig2,Heinritzi Martin4,Holanda Bruna A.2,Jöckel Patrick3,Kaiser Katharina9,Krüger Ovid O.2,Lucke Johannes10,Marsing Andreas3,Martin Anna2,Matthes Sigrun3,Pöhlker Christopher2,Pöschl Ulrich2,Reifenberg Simon2,Ringsdorf Akima2,Scheibe Monika3,Tadic Ivan2,Zauner-Wieczorek Marcel4,Henke Rolf3,Rapp Markus11

Affiliation:

1. Deutsches Zentrum für Luft- und Raumfahrt, Oberpfaffenhofen, and Johannes Gutenberg-Universität, Mainz, Germany;

2. Max-Planck-Institut für Chemie, Mainz, Germany;

3. Deutsches Zentrum für Luft- und Raumfahrt, Oberpfaffenhofen, Germany;

4. Goethe-Universität Frankfurt, Frankfurt, Germany;

5. Forschungszentrum Jülich, Jülich, Germany;

6. Max-Planck-Institut für Chemie, Mainz, and Leipzig Institut für Meteorologie, Universität Leipzig, and Leibniz Institut für Troposphärenforschung, Leipzig, Germany;

7. Karlsruhe Institut für Technologie, Karlsruhe, Germany;

8. Max-Planck-Institut für Chemie, Mainz, Germany, and Scripps Institution of Oceanography, University of California, San Diego, La Jolla, California;

9. Johannes Gutenberg-Universität, and Max-Planck-Institut für Chemie, Mainz, Germany;

10. Deutsches Zentrum für Luft- und Raumfahrt, Oberpfaffenhofen, Germany, and Faculty of Aerospace Engineering, Delft University of Technology, Delft, Netherlands;

11. Deutsches Zentrum für Luft- und Raumfahrt, Oberpfaffenhofen, and Ludwig-Maximilians-Universität, Munich, Germany

Abstract

Abstract During spring 2020, the COVID-19 pandemic caused massive reductions in emissions from industry and ground and airborne transportation. To explore the resulting atmospheric composition changes, we conducted the BLUESKY campaign with two research aircraft and measured trace gases, aerosols, and cloud properties from the boundary layer to the lower stratosphere. From 16 May to 9 June 2020, we performed 20 flights in the early COVID-19 lockdown phase over Europe and the Atlantic Ocean. We found up to 50% reductions in boundary layer nitrogen dioxide concentrations in urban areas from GOME-2B satellite data, along with carbon monoxide reductions in the pollution hot spots. We measured 20%–70% reductions in total reactive nitrogen, carbon monoxide, and fine mode aerosol concentration in profiles over German cities compared to a 10-yr dataset from passenger aircraft. The total aerosol mass was significantly reduced below 5 km altitude, and the organic aerosol fraction also aloft, indicative of decreased organic precursor gas emissions. The reduced aerosol optical thickness caused a perceptible shift in sky color toward the blue part of the spectrum (hence BLUESKY) and increased shortwave radiation at the surface. We find that the 80% decline in air traffic led to substantial reductions in nitrogen oxides at cruise altitudes, in contrail cover, and in resulting radiative forcing. The light extinction and depolarization by cirrus were also reduced in regions with substantially decreased air traffic. General circulation–chemistry model simulations indicate good agreement with the measurements when applying a reduced emission scenario. The comprehensive BLUESKY dataset documents the major impact of anthropogenic emissions on the atmospheric composition.

Publisher

American Meteorological Society

Subject

Atmospheric Science

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