The fluctuation–dissipation measurement instrument at the Linac Coherent Light Source

Author:

Assefa T. A.12,Seaberg M. H.3ORCID,Reid A. H.3ORCID,Shen L.12,Esposito V.1,Dakovski G. L.3,Schlotter W.3,Holladay B.34,Streubel R.56ORCID,Montoya S. A.7,Hart P.3ORCID,Nakahara K.3,Moeller S.3ORCID,Kevan S. D.89ORCID,Fischer P.5ORCID,Fullerton E. E.710,Colocho W.3ORCID,Lutman A.3ORCID,Decker F.-J.3ORCID,Sinha S. K.4,Roy S.9,Blackburn E.2ORCID,Turner J. J.13ORCID

Affiliation:

1. Stanford Institute for Materials and Energy Science, Stanford University and SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA

2. Division of Synchrotron Radiation Research, Department of Physics, Lund University, 22100 Lund, Sweden

3. Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, California 94720, USA

4. Department of Physics, University of California—San Diego, La Jolla, California 92093, USA

5. Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA and Physics Department, University of California Santa Cruz, Santa Cruz, California 95064, USA

6. Department of Physics and Astronomy and Nebraska Center for Materials and Nanoscience, University of Nebraska-Lincoln, Lincoln, Nebraska 68588, USA

7. Center for Memory and Recording Research, University of California—San Diego, La Jolla, California 92093, USA

8. Department of Physics, University of Oregon, Eugene, Oregon 97401, USA

9. Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA

10. Department of Electrical and Computer Engineering, University of California—San Diego, La Jolla, California 92093, USA

Abstract

The development of new modes at x-ray free electron lasers has inspired novel methods for studying fluctuations at different energies and timescales. For closely spaced x-ray pulses that can be varied on ultrafast time scales, we have constructed a pair of advanced instruments to conduct studies targeting quantum materials. We first describe a prototype instrument built to test the proof-of-principle of resonant magnetic scattering using ultrafast pulse pairs. This is followed by a description of a new endstation, the so-called fluctuation–dissipation measurement instrument, which was used to carry out studies with a fast area detector. In addition, we describe various types of diagnostics for single-shot contrast measurements, which can be used to normalize data on a pulse-by-pulse basis and calibrate pulse amplitude ratios, both of which are important for the study of fluctuations in materials. Furthermore, we present some new results using the instrument that demonstrates access to higher momentum resolution.

Funder

U.S. Department of Energy

U.S. Office of Naval Research National Science Foundation/EPSCoR RII Track-1: Emergent Quantum Materials and Technologies

Publisher

AIP Publishing

Subject

Instrumentation

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