Compression rate of dynamic diamond anvil cells from room temperature to 10 K

Abstract

There is an ever increasing interest in studying dynamic-pressure dependent phenomena utilizing dynamic Diamond Anvil Cells (dDACs), devices capable of a highly controlled rate of compression. Here, we characterize and compare the compression rate of dDACs in which the compression is actuated via three different methods: (1) stepper motor (S-dDAC), (2) gas membrane (M-dDAC), and (3) piezoactuator (P-dDAC). The compression rates of these different types of dDAC were determined solely on millisecond time-resolved R1-line fluorescence of a ruby sphere located within the sample chamber. Furthermore, these different dynamic compression-techniques have been described and characterized over a broad temperature and pressure range from 10 to 300 K and 0–50 GPa. At room temperature, piezoactuation (P-dDAC) has a clear advantage in controlled extremely fast compression, having recorded a compression rate of ∼7 TPa/s, which is also found to be primarily influenced by the charging time of the piezostack. At 40–250 K, gas membranes (M-dDAC) have also been found to generate rapid compression of ∼0.5–3 TPa/s and are readily interfaced with moderate cryogenic and ultrahigh vacuum conditions. Approaching more extreme cryogenic conditions (<10 K), a stepper motor driven lever arm (S-dDAC) offers a solution for high-precision moderate compression rates in a regime where P-dDACs and M-dDACs can become difficult to incorporate. The results of this paper demonstrate the applicability of different dynamic compression techniques, and when applied, they can offer us new insights into matter’s response to strain, which is highly relevant to physics, geoscience, and chemistry.