Collective dynamics in a glass-former with Mari–Kurchan interactions

Author:

Nishikawa Yoshihiko12ORCID,Ikeda Atsushi3ORCID,Berthier Ludovic14ORCID

Affiliation:

1. Laboratoire Charles Coulomb (L2C), Université de Montpellier, CNRS, 34095 Montpellier, France

2. Graduate School of Information Sciences, Tohoku University, Sendai 980-8579, Japan

3. Graduate School of Arts and Sciences, The University of Tokyo, Tokyo 153-8902, Japan

4. Yusuf Hamied Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2 1EW, United Kingdom

Abstract

We numerically study the equilibrium relaxation dynamics of a two-dimensional Mari–Kurchan glass model. The tree-like structure of particle interactions forbids both nontrivial structural motifs and the emergence of a complex free-energy landscape leading to a thermodynamic glass transition, while the finite-dimensional nature of the model prevents the existence of a mode-coupling singularity. Nevertheless, the equilibrium relaxation dynamics is shown to be in excellent agreement with simulations performed in conventional glass-formers. Averaged time correlation functions display a phenomenology typical of supercooled liquids, including the emergence of an excess signal in relaxation spectra at intermediate frequencies. We show that this evolution is accompanied by strong signatures of collective and heterogeneous dynamics that cannot be interpreted in terms of single particle hopping and emerge from dynamic facilitation. Our study demonstrates that an off-lattice interacting particle model with extremely simple structural correlations displays quantitatively realistic glassy dynamics.

Funder

Simons Foundation

Japan Society for the Promotion of Science London

Publisher

AIP Publishing

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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