Sub-100-picosecond time resolution from undoped and Li-doped two-dimensional perovskite scintillators

Author:

Cala' Roberto1ORCID,Frank Isabel1,Pagano Fiammetta1ORCID,Maddalena Francesco2ORCID,Dang Cuong2ORCID,Birowosuto Muhammad Danang3ORCID,Auffray Etiennette1ORCID

Affiliation:

1. CERN, Esplanade des Particules 1, 1211 Meyrin, Switzerland

2. CINTRA UMI CNRS/NTU/THALES 3288, Research Techno Plaza, 50 Nanyang Drive, Border X Block, Level 6, Singapore 637553, Singapore

3. Łukasiewicz Research Network-PORT Polish Center for Technology Development, Stabłowicka 147, 54-066 Wrocław, Poland

Abstract

Fast hybrid organic–inorganic two-dimensional (2D) perovskite scintillators with high light yield are measured for their scintillating properties. With a light yield of 17 300 ± 2140 photons/MeV, undoped PEA2PbBr4 crystals already exhibit 100 ± 4 ps coincidence time resolution (CTR) at 511 keV excitation. However, Li-doped PEA2PbBr4 crystals have improved the light yield to 21 400 ± 2140 photons/MeV and showed sub-100 ps CTR. Such CTR values and low-cost manufacturing processes make these 2D perovskite scintillators as promising competitors for commercial lanthanide scintillators in time-of-flight positron emission tomography and for fast timing detectors.

Funder

Ministry of Education - Singapore

Publisher

AIP Publishing

Subject

Physics and Astronomy (miscellaneous)

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