Correlation functions from tensor network influence functionals: The case of the spin-boson model

Author:

Nguyen Haimi1ORCID,Ng Nathan1ORCID,Lindoy Lachlan P.2ORCID,Park Gunhee3ORCID,Millis Andrew J.45ORCID,Kin-Lic Chan Garnet6ORCID,Reichman David R.1ORCID

Affiliation:

1. Department of Chemistry, Columbia University 1 , New York, New York 10027, USA

2. National Physical Laboratory 2 , Teddington TW11 0LW, United Kingdom

3. Division of Engineering and Applied Science, California Institute of Technology 3 , Pasadena, California 91125, USA

4. Department of Physics, Columbia University 4 , New York, New York 10027, USA

5. Center for Computational Quantum Physics, Flatiron Institute 5 , New York, New York 10010, USA

6. Division of Chemistry and Chemical Engineering, California Institute of Technology 6 , Pasadena, California 91125, USA

Abstract

We investigate the application of matrix product state (MPS) representations of the influence functionals (IFs) for the calculation of real-time equilibrium correlation functions in open quantum systems. Focusing specifically on the unbiased spin-boson model, we explore the use of IF-MPSs for complex time propagation, as well as IF-MPSs for constructing correlation functions in the steady state. We examine three different IF approaches: one based on the Kadanoff–Baym contour targeting correlation functions at all times, one based on a complex contour targeting the correlation function at a single time, and a steady state formulation, which avoids imaginary or complex times, while providing access to correlation functions at all times. We show that within the IF language, the steady state formulation provides a powerful approach to evaluate equilibrium correlation functions.

Funder

U.S. Department of Energy

Engineering and Physical Sciences Research Council

Publisher

AIP Publishing

Reference64 articles.

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