Enhanced photoconductivity of hybrid 2D-QD MoS2–AgInS2 structures

Author:

Kondratenko Serhiy1ORCID,Datsenko Oleksandr I.1ORCID,Babich Danylo1ORCID,Dzhagan Volodymyr12ORCID,Pan Yang34ORCID,Rahaman Mahfujur3ORCID,Selyshchev Oleksandr34ORCID,Zahn Dietrich R. T.34ORCID

Affiliation:

1. Taras Shevchenko National University of Kyiv 1 , 64 Volodymyrs’ka St., 01601 Kyiv, Ukraine

2. V.E. Lashkaryov Institute of Semiconductors Physics, NAS of Ukraine 2 , 41 pr. Nauki, 03028 Kyiv, Ukraine

3. Semiconductor Physics, Chemnitz University of Technology 3 , 09107 Chemnitz, Germany

4. Center for Materials, Architectures and Integration of Nanomembranes (MAIN), Chemnitz University of Technology 4 , 09107 Chemnitz, Germany

Abstract

This study describes the fabrication of hybrid two-dimensional (2D)-quantum dot (QD) MoS2–AgInS2 photoconductive devices through the mechanical pressing of a MoS2 flake onto an AgInS2 QD film. The devices exhibit an enhanced photoresponse at both continuous and modulated optical excitations, compared with the bare MoS2 or AgInS2 layer, due to the formation of a built-in electric field near the MoS2/AgInS2 interface. The continuous wave photoresponse is significantly higher due to the effective photoconductive gain when electrons flow freely through the MoS2 flake, whereas holes are effectively trapped in AgInS2 QDs. The study highlights the potential of hybrid 2D-QD MoS2–AgInS2 devices for photovoltaic and optoelectronic applications.

Funder

National Research Foundation of Ukraine

Deutsche Forschungsgemeinschaft

Publisher

AIP Publishing

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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