X-ray investigation of long-range antiferromagnetic ordering in FeRh

Author:

Grimes M.123ORCID,Gurung N.23,Ueda H.2ORCID,Porter D. G.4ORCID,Pedrini B.2,Heyderman L. J.23ORCID,Thomson T.1ORCID,Scagnoli V.23

Affiliation:

1. NEST, Department of Computer Science, The University of Manchester, Oxford Road, Manchester M13 9PL, United Kingdom

2. Paul Scherrer Institute, 5232 Villigen PSI, Switzerland

3. Laboratory for Mesoscopic Systems, Department of Materials, ETH Zurich, 8093 Zurich, Switzerland

4. Diamond Light Source, Harwell Science and Innovation Campus, Didcot OX11 0DE, United Kingdom

Abstract

We demonstrate a probe of long-range antiferromagnetic (AF) order in FeRh thin films using non-resonant magnetic x-ray scattering. In particular, x-rays at energies below the Fe K-edge have been used for the observation of magnetic Bragg peaks. Due to the low efficiency of the magnetic scattering, a grazing incidence geometry was used to optimise the diffracted intensity from the thin film samples. Based on Scherrer analysis, we estimate a coherence length similar to previous reports from x-ray magnetic linear dichroism (XMLD) experiments, indicating that domain sizes are limited to 40 nm which is consistent with the grain size. The temperature dependent behaviour of the AF order shows an inverse correlation with the emergence of the ferromagnetic (FM) moment, as expected from the phase diagram.

Funder

Faculty of Science and Engineering, University of Manchester

Paul Scherrer Institut

Diamond Light Source

Henry Royce Institute

Swiss National Science Foundation

H2020 Marie Skłodowska-Curie Actions

National Centers of Competence in Research in Molecular Ultrafast Science and Technology

Publisher

AIP Publishing

Subject

General Physics and Astronomy

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