An overview of the spin dynamics of antiferromagnetic Mn5Si3

Author:

Biniskos N.12ORCID,dos Santos F. J.34ORCID,dos Santos Dias M.567ORCID,Raymond S.8ORCID,Schmalzl K.9ORCID,Steffens P.10,Persson J.11,Marzari N.34ORCID,Blügel S.5ORCID,Lounis S.56ORCID,Brückel T.11ORCID

Affiliation:

1. Forschungszentrum Jülich GmbH, Jülich Centre for Neutron Science at MLZ 1 , Lichtenbergstr. 1, D-85748 Garching, Germany

2. Charles University, Faculty of Mathematics and Physics, Department of Condensed Matter Physics 2 , Ke Karlovu 5, 121 16 Praha, Czech Republic

3. Laboratory for Materials Simulations, Paul Scherrer Institut 3 , 5232 Villigen PSI, Switzerland

4. Theory and Simulation of Materials (THEOS), and National Centre for Computational Design and Discovery of Novel Materials (MARVEL), École Polytechnique Fédérale de Lausanne 4 , 1015 Lausanne, Switzerland

5. Peter Grünberg Institut and Institute for Advanced Simulation, Forschungszentrum Jülich & JARA 5 , D-52425 Jülich, Germany

6. Faculty of Physics, University of Duisburg-Essen and CENIDE 6 , D-47053 Duisburg, Germany

7. Scientific Computing Department, STFC Daresbury Laboratory 7 , Warrington WA4 4AD, United Kingdom

8. Université Grenoble Alpes, CEA, IRIG, MEM, MDN 8 , F-38000 Grenoble, France

9. Forschungszentrum Jülich GmbH, Jülich Centre for Neutron Science at ILL 9 , 71 Avenue des Martyrs, F-38000 Grenoble, France

10. Institut Laue-Langevin 10 , 71 Avenue des Martyrs, 38000 Grenoble, France

11. Forschungszentrum Jülich GmbH, Jülich Centre for Neutron Science (JCNS-2) and Peter Grünberg Institut (PGI-4), JARA-FIT 11 , D-52425 Jülich, Germany

Abstract

The metallic compound Mn5Si3 hosts a series of antiferromagnetic phases that can be controlled by external stimuli, such as temperature and magnetic field. In this work, we investigate the spin-excitation spectrum of bulk Mn5Si3 by combining inelastic neutron scattering measurements and density functional theory calculations. We study the evolution of the dynamical response under external parameters and demonstrate that the spin dynamics of each phase is robust against any combination of temperature and magnetic field. In particular, the high-energy spin dynamics is very characteristic of the different phases consisting of either spin waves or broad fluctuation patterns.

Funder

Grantová Agentura České Republiky

H2020 Industrial Leadership

Coordenação de Aperfeiçoamento de Pessoal de Nível Superior

Deutsche Forschungsgemeinschaft

Publisher

AIP Publishing

Subject

General Engineering,General Materials Science

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