Destruction of a magnesium alloy film in the condensed state by an ultrashort laser-driven shock wave

Abstract

Laser-driven shock wave phenomena in a sub-micrometer Mg–4Al–2Zn alloy film are studied using spectral interferometry with spatial and temporal (1 ps) resolution. Upon irradiating the film through a glass substrate by 500 fs laser pulses, the ultrashort elastic compression pulses with the peak stress up to 4.6 GPa at a propagation distance of 0.5 μm were generated. Depending on the laser fluence, either spall fracture near the rear surface in the solid state or cavitation near the metal–glass interface in the liquid state was observed. The spall strength of the solid Mg alloy and the upper limit of the cavitation threshold in the melt at the strain rate of ∼109 s−1 were extracted from the free surface velocity history. The depth of fracture initiation was retrieved from the instant of the spall pulse exit, and the thickness of the molten layer was estimated to be 100–160 nm depending on laser fluence. The investigation of the residual morphology by scanning electron and atomic force microscopies revealed the presence of melting and nucleation within the irradiated area. The experimental findings are of interest for predicting the behavior of magnesium alloys in the condensed state at extremely high strain rates, for studying the physics of metastable states and for simulating the interaction of ultrashort laser pulses with thin film materials.