Optical spectrum of n-type and p-type monolayer MoS2 in the presence of proximity-induced interactions

Author:

Liu J.1ORCID,Xu W.123ORCID,Xiao Y. M.1ORCID,Ding L.1ORCID,Li H. W.2ORCID,Peeters F. M.24ORCID

Affiliation:

1. School of Physics and Astronomy and Yunnan Key Laboratory of Quantum Information, Yunnan University 1 , Kunming 650091, China

2. Micro Optical Instruments Inc. 2 , Shenzhen 518118, China

3. Key Laboratory of Materials Physics, Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences, HFIPS 3 , Hefei 230031, China

4. Department of Physics, University of Antwerp 4 , Groenenborgerlaan 171, B-2020 Antwerpen, Belgium

Abstract

In this paper, we examined the effects of proximity-induced interactions such as Rashba spin-orbit coupling and effective Zeeman fields (EZFs) on the optical spectrum of n-type and p-type monolayer (ML)-MoS2. The optical conductivity is evaluated using the standard Kubo formula under random-phase approximation by including the effective electron–electron interaction. It has been found that there exist two absorption peaks in n-type ML-MoS2 and two knife shaped absorptions in p-type ML-MoS2, which are contributed by the inter-subband spin-flip electronic transitions within conduction and valence bands at valleys K and K′ with a lifted valley degeneracy. The optical absorptions in n-type and p-type ML-MoS2 occur in THz and infrared radiation regimes and the position, height, and shape of them can be effectively tuned by Rashba parameter, EZF parameters, and carrier density. The interesting theoretical predictions in this study would be helpful for the experimental observation of the optical absorption in infrared to THz bandwidths contributed by inter-subband spin-flip electronic transitions in a lifted valley degeneracy monolayer transition metal dichalcogenides system. The obtained results indicate that ML-MoS2 with the platform of proximity interactions make it a promising infrared and THz material for optics and optoelectronics.

Funder

National Natural Science Foundation of China

Shenzhen Science and Technology Innovation Program

Applied Basic Research Foundation of Yunnan Province

People's Government of Yunnan Province

Publisher

AIP Publishing

Subject

General Physics and Astronomy

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