Dynamical anomalies and structural features of active Brownian particles characterized by two repulsive length scales

Author:

Martín-Roca José1ORCID,Martinez Raúl12,Martínez-Pedrero Fernando3,Ramírez Jorge4ORCID,Valeriani Chantal15ORCID

Affiliation:

1. Dep. de Est. de la Materia, Física Térmica y Electrónica, Universidad Complutense de Madrid, 28040 Madrid, Spain

2. Dep. de Física Teórica de la Materia Condensada, Facultad de Ciencias, Universidad Autónoma de Madrid, 28049 Madrid, Spain

3. Dep. Química-Fiśica, Universidad Complutense de Madrid, Avda. Complutense s/n, Madrid 28040, Spain

4. Dep. de Ingeniería Química, ETSI Industriales, Universidad Politécnica de Madrid, 28006 Madrid, Spain

5. GISC - Grupo Interdisciplinar de Sistemas Complejos, 28040 Madrid, Spain

Abstract

In this work, we study a two-dimensional system composed by Active Brownian Particles (ABPs) interacting via a repulsive potential with two length scales—a soft shell and a hard core. Depending on the ratio between the strength of the soft shell barrier and the activity, we find two regimes: If this ratio is much larger or smaller than 1, the observed behavior is comparable with ABPs interacting via a single length scale potential. If this ratio is similar to 1, the two length scales are relevant for both structure and dynamical properties. On the structural side, when the system exhibits a motility induced phase separation, the dense phase is characterized by new and more complex structures compared with the hexatic phase observed in single length scale systems. From the dynamic analysis, we find, to our knowledge, the first manifestation of a dynamic heterogeneity in active particles, reminiscent of the glassy dynamics widely studied in passive colloids.

Funder

Ministerio de Asuntos Económicos y Transformación Digital, Gobierno de España

Publisher

AIP Publishing

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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