Pressure-cycling induced transition behaviors of MnBi2Te4

Author:

Wu Jie12ORCID,Feng Yan3ORCID,Ren Yifeng2,Zhang Ziyou1ORCID,Yang Yanping1ORCID,Wang Xinyao45ORCID,Su Fuhai5ORCID,Dong Hongliang1ORCID,Lu Yang1,Zhang Xiaojun6,Deng Yu2ORCID,Xiang Bin3ORCID,Chen Zhiqiang1ORCID

Affiliation:

1. Center for High Pressure Science and Technology Advanced Research 1 , Shanghai 201203, China

2. National Laboratory of Solid State Microstructure, School of Physics, Nanjing University 2 , Nanjing 210093, China

3. Department of Materials Science and Engineering, CAS Key Lab of Materials for Energy Conversion, Anhui Laboratory of Advanced Photon Science and Technology, University of Science and Technology of China 3 , Hefei 230026, China

4. University of Science and Technology of China 4 , Hefei 230026, China

5. Key Laboratory of Materials Physics, Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences 5 , Hefei 230031, China

6. Arrayed Materials (China) Co., Ltd. 6 , Shenzhen 518000, China

Abstract

MnBi2Te4 can generate a variety of exotic topological quantum states, which are closely related to its special structure. We conduct comprehensive multiple-cycle high-pressure research on MnBi2Te4 by using a diamond anvil cell to study its phase transition behaviors under high pressure. As observed, when the pressure does not exceed 15 GPa, the material undergoes an irreversible metal–semiconductor–metal transition, whereas when the pressure exceeds 17 GPa, the layered structure is damaged and becomes irreversibly amorphous due to the lattice distortion caused by compression, but it is not completely amorphous, which presents some nano-sized grains after decompression. Our investigation vividly reveals the phase transition behaviors of MnBi2Te4 under high pressure cycling and paves the experimental way to find topological phases under high pressure.

Funder

NSAF Joint Fund

Innovation Program for Quantum Science and Technology

National Natural Science Foundation of China

Natural Science Foundation of Jiangsu Province

Publisher

AIP Publishing

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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