Using tensor network states for multi-particle Brownian ratchets

Author:

Strand Nils E.1ORCID,Vroylandt Hadrien1ORCID,Gingrich Todd R.1ORCID

Affiliation:

1. Department of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208, USA

Abstract

The study of Brownian ratchets has taught how time-periodic driving supports a time-periodic steady state that generates nonequilibrium transport. When a single particle is transported in one dimension, it is possible to rationalize the current in terms of the potential, but experimental efforts have ventured beyond that single-body case to systems with many interacting carriers. Working with a lattice model of volume-excluding particles in one dimension, we analyze the impact of interactions on a flashing ratchet’s current. To surmount the many-body problem, we employ the time-dependent variational principle applied to binary tree tensor networks. Rather than propagating individual trajectories, the tensor network approach propagates a distribution over many-body configurations via a controllable variational approximation. The calculations, which reproduce Gillespie trajectory sampling, identify and explain a shift in the frequency of maximum current to higher driving frequency as the lattice occupancy increases.

Funder

National Science Foundation

Publisher

AIP Publishing

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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