Author:
Chen F. -R.,Kisielowski C.,Van Dyck D.
Abstract
AbstractIt is now established that the 3D structure of homogeneous nanocrystals can be recovered from in-line hologram of single projections. The method builds on a quantitative contrast interpretation of electron exit wave functions. Since simulated exit wave functions of single and bilayers of graphene reveal the atomic structure of carbon-based materials with sufficient resolution, we explore theoretically how the approach can be expanded beyond periodic carbon-based materials to include non-periodic molecular structures. We show here theoretically that the 3D atomic structure of randomly oriented oleic acid molecules can be recovered from a single projection.
Funder
NSC
U.S. Department of Energy
the Fund for Scientific Research - Flanders
Publisher
Springer Science and Business Media LLC
Subject
Spectroscopy,Radiology Nuclear Medicine and imaging,Chemical Engineering (miscellaneous)
Reference14 articles.
1. Van Aert, S., Batenburg, K.J., Rossell, M.D., Erni, R., Van Tendeloo, G.: Three-dimensional atomic imaging of crystalline nanoparticles. Nature 374, 470 (2011)
2. Scott, M.C., Chen, C.C., Mecklenburg, M., Zhu, C., Xu, R., Ercius, P., Dahmen, U., Regan, B.C., Miao, J.: Electron tomography at 2.4-ångström resolution. Nature 483, 444–447 (2012)
3. Van Dyck, D., Jinschek, J.R., Chen, F.R.: Big-Bang tomography as a new route to atomic resolution electron tomography. Nature 486, 243 (2012)
4. Chen, F.-R., Van Dyck, D., Kisielowski, C.: In-line three-dimensional holography of nanocrystalline objects at atomic resolution. Nat. Commun. 7, 10603 (2016)
5. Coene, W., Thust, A., Van Dyck, D., de Beeck, M.: Maximum-likelihood method for focus-variation image reconstruction in high resolution transmission electron microscopy. Ultramicroscopy 64, 109–135 (1996)
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