Affiliation:
1. School of Atmospheric Sciences Joint International Research Laboratory of Atmospheric and Earth System Sciences Jiangsu Provincial Collaborative Innovation Center of Climate Change Nanjing University Nanjing China
2. Frontiers Science Center for Critical Earth Material Cycling Nanjing University Nanjing China
3. Pacific Northwest National Laboratory Richland WA USA
4. School of Environmental Science and Engineering Southern University of Science and Technology Shenzhen China
5. Department of Chemistry and Department of Environmental and Molecular Toxicology Oregon State University Corvallis OR USA
6. Pacific Northwest National Laboratory Joint Global Change Research Institute College Park MD USA
7. Laboratory for Earth Surface Processes College of Urban and Environmental Sciences Peking University Beijing China
Abstract
AbstractLung cancer risk from exposure to ambient polycyclic aromatic hydrocarbons (PAHs) is expected to change significantly by 2050 compared to 2008 due to changes in climate and emissions. Integrating a global atmospheric chemistry model, a lung cancer risk model, and plausible future emissions trajectories of PAHs, we assess how global PAHs and their associated lung cancer risk will likely change in the future. Benzo(a)pyrene (BaP) is used as an indicator of cancer risk from PAH mixtures. From 2008 to 2050, the population‐weighted global average BaP concentrations under all RCPs consistently exceeded the WHO‐recommended limits, primarily attributed to residential biofuel use. Peaks in PAH‐associated incremental lifetime cancer risk shift from East Asia (4 × 10−5) in 2008 to South Asia (mostly India, 2–4 × 10−5) and Africa (1–2 × 10−5) by 2050. In the developing regions of Africa and South Asia, PAH‐associated lung cancer risk increased by 30–64% from 2008 to 2050, due to increasing residential energy demand in households for cooking, heating, and lighting, the continued use of traditional biomass use, increases in agricultural waste burning, and forest fires, accompanied by rapid population growth in these regions. Due to more stringent air quality policies in developed countries, their PAH lung cancer risk substantially decreased by ∼80% from 2008 to 2050. Climate change is likely to have minor effects on PAH lung cancer risk compared to the impact of emissions. Future policies, therefore, need to consider efficient combustion technologies that reduce air pollutant emissions, including incomplete combustion products such as PAH.
Publisher
American Geophysical Union (AGU)
Subject
Earth and Planetary Sciences (miscellaneous),General Environmental Science
Cited by
2 articles.
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