On the origin of129I in rain water near Zürich

Abstract

129I concentrations in precipitation at Dübendorf/Zürich, Switzerland, have been determined with monthly resolution for almost three years in the mid 1990s. The results confirm that annual mean129I concentrations in precipitation in central Europe have remained about constant since the late 1980s. Liquid and gaseous emissions from the nuclear fuel reprocessing plants at Sellafield and La Hague are discussed as the only possible sources of129I in precipitation in central Europe. Based on an upper limit estimate for iodine transferred from the sea to the atmosphere, the gaseous discharges constitute the potentially bigger129I reservoir for precipitation. Moreover, the time dependence of the annual gaseous129I releases from Sellafield and La Hague correlates much better with the129I concentrations in precipitation in central Europe since the late 1980s than does the time dependence of the liquid emissions from these sites. At monthly resolution, the129I concentrations in the precipitation samples close to Zürich exhibit a large variability. A meteorological transport analysis was carried out for four selected months with particularly low or high observed129I concentrations. It was found that meteorological transport alone, based upon assimilated wind fields and observed precipitation values, can not directly account for the large month-to-month variability.