Soft X-Ray Phase Nanomicroscopy of Micrometer-Thick Magnets

Abstract

Imaging of nanoscale magnetic textures within extended material systems is of critical importance to both fundamental research and technological applications. While high-resolution magnetic imaging of thin nanoscale samples is well established with electron and soft x-ray microscopy, the extension to micrometer-thick systems currently requires hard x rays, which limits high-resolution imaging to rare-earth magnets. Here, we overcome this limitation by establishing soft x-ray magnetic imaging of micrometer-thick systems using the pre-edge phase x-ray magnetic circular dichroism signal, thus making possible the study of a wide range of magnetic materials. By performing dichroic spectroptychography, we demonstrate high spatial resolution imaging of magnetic samples up to 1.7  μm thick, an order of magnitude higher than conventionally possible with soft x-ray absorption-based techniques. We demonstrate the applicability of the technique by harnessing the pre-edge phase to image thick chiral helimagnets, and naturally occurring magnetite particles, gaining insight into their three-dimensional magnetic configuration. This new regime of magnetic imaging makes possible the study of extended non-rare-earth systems that have until now been inaccessible, including magnetic textures for future spintronic applications, non-rare-earth permanent magnets for energy harvesting, and the magnetic configuration of giant magnetofossils. Published by the American Physical Society 2024