Multi-angle tracking synthetic kinetics of phase evolution in Li-rich Mn-based cathodes

Author:

Xu Shenyang1ORCID,Chen Zhefeng1,Zhao Wenguang1,Ren Wenju12,Hou Chenxin1,Liu Jiajie1,Wang Wu3,Yin Chong4,Tan Xinghua1,Lou Xiaobing5ORCID,Yao Xiangming1,Gao Zhihai1,Liu Hao6,Wang Lu1,Yin Zuwei1ORCID,Qiu Bao7ORCID,Hu Bingwen5ORCID,Li Tianyi8ORCID,Dong Cheng1ORCID,Pan Feng1ORCID,Zhang Mingjian9

Affiliation:

1. School of Advanced Materials, Shenzhen Graduate School, Peking University, Shenzhen 518055, China

2. School of Advanced Manufacturing Engineering, Chongqing University of Posts and Telecommunications, Chongqing 400065, China

3. Shenzhen Key Laboratory of Thermoelectric Materials, Department of Physics, Southern University of Science and Technology, Shenzhen 518055, China

4. Ningbo Ronbay Lithium Battery Material Co., Ltd, Ningbo 315400, China

5. Shanghai Key Laboratory of Magnetic Resonance, State Key Laboratory of Precision Spectroscopy, School of Physics and Electronic Science, East China Normal University, Shanghai 200241, China

6. Institute for Applied Materials, Karlsruhe Institute of Technology, Hermann-von-Helmholtz-Platz 1, Eggenstein-Leopoldshafen 76344, Germany

7. Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, China

8. Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, IL 60439, USA

9. School of Science and Engineering, The Chinese University of Hong Kong, Shenzhen, Guangdong 518172, China

Abstract

This study investigates the two-phase fusion in Li-rich Mn-based cathodes, revealing the process from two-phase formation to solid solution, and optimizes performance by controlling the fusion extent in lithium and sodium cathode materials.

Funder

National Natural Science Foundation of China-Guangdong Joint Fund

Shenzhen Key Laboratory of Eco-materials and Renewable Energy

Basic and Applied Basic Research Foundation of Guangdong Province

Publisher

Royal Society of Chemistry (RSC)

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