Time-resolved observation of transient precursor state of CO on Ru(0001) using carbon K-edge spectroscopy

Author:

Wang Hsin-Yi12345ORCID,Schreck Simon12345,Weston Matthew12345,Liu Chang12345ORCID,Ogasawara Hirohito678,LaRue Jerry910118,Perakis Fivos12345ORCID,Dell’Angela Martina121314ORCID,Capotondi Flavio15161314,Giannessi Luca15161314,Pedersoli Emanuele15161314,Naumenko Denys15161314,Nikolov Ivaylo15161314,Raimondi Lorenzo15161314,Spezzani Carlo15161314,Beye Martin171819,Cavalca Filippo12345,Liu Boyang12345,Gladh Jörgen12345ORCID,Koroidov Sergey12345,Miedema Piter S.171819,Costantini Roberto1213142021ORCID,Pettersson Lars G. M.12345,Nilsson Anders12345ORCID

Affiliation:

1. Department of Physics

2. AlbaNova University Center

3. Stockholm University

4. SE-10691 Stockholm

5. Sweden

6. SLAC National Accelerator Laboratory

7. Menlo Park

8. USA

9. Schmid College of Science and Technology

10. Chapman University

11. Orange

12. CNR-IOM

13. Trieste

14. Italy

15. FERMI

16. Elettra-Sincrotrone Trieste

17. DESY Photon Science

18. Hamburg 22607

19. Germany

20. Physics Department

21. University of Trieste

Abstract

The transient dynamics of carbon monoxide (CO) molecules on a Ru(0001) surface following femtosecond optical laser pump excitation has been studied by monitoring changes in the unoccupied electronic structure using an ultrafast X-ray free-electron laser (FEL) probe.

Funder

Vetenskapsrådet

Knut och Alice Wallenbergs Stiftelse

Helmholtz Association

Ministero dell’Istruzione, dell’Università e della Ricerca

Basic Energy Sciences

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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