Highly efficient and selective aqueous phase hydrogenation of aryl ketones, aldehydes, furfural and levulinic acid and its ethyl ester catalyzed by phosphine oxide-decorated polymer immobilized ionic liquid-stabilized ruthenium nanoparticles-Reference-Cited by-同舟云学术

Highly efficient and selective aqueous phase hydrogenation of aryl ketones, aldehydes, furfural and levulinic acid and its ethyl ester catalyzed by phosphine oxide-decorated polymer immobilized ionic liquid-stabilized ruthenium nanoparticles

Published:2022 Issue:11 Volume:12 Page:3549-3567
ISSN:2044-4753
Container-title:Catalysis Science & Technology
language:en
Short-container-title:Catal. Sci. Technol.

Author:

Doherty S.¹^ORCID,Knight J. G.¹^ORCID,Backhouse T.¹,Tran T. S. T.¹,Paterson R.¹,Stahl F.¹,Alharbi H. Y.¹,Chamberlain T. W.²^ORCID,Bourne R. A.²^ORCID,Stones R.²,Griffiths A.²,White J. P.²,Aslam Z.²,Hardare C.³^ORCID,Daly H.³^ORCID,Hart J.⁴,Temperton R. H.⁴,O'Shea J. N.⁴,Rees N. H.⁵^ORCID

Affiliation:

1. Newcastle University Centre for Catalysis (NUCAT), School of Chemistry, Bedson Building, Newcastle University, Newcastle upon Tyne, NE1 7RU, UK

2. Institute of Process Research & Development, School of Chemistry and School of Chemical and Process Engineering, University of Leeds, Woodhouse Land Leeds, LS2 9JT, UK

3. School of Chemical Engineering and Analytical Sciences, The University of Manchester, The Mill, Sackville Street Campus, Manchester, M13 9PL, UK

4. School of Physics & Astronomy, University of Nottingham, Nottingham, NG7 2RD, UK

5. Inorganic Chemistry Laboratory, University of Oxford, South Parks Road, Oxford OX1 3QR, UK

Abstract

Phosphine oxide-decorated polymer immobilized ionic liquid stabilized RuNPs catalyse the hydrogenation of aryl ketones with remarkable selectivity for the CO bond, complete hydrogenation to the cyclohexylalcohol and hydrogenation of levulinic acid to γ-valerolactone.

Funder

Engineering and Physical Sciences Research Council

Newcastle University

Taibah University

Publisher

Royal Society of Chemistry (RSC)

Subject

Catalysis

Link

http://pubs.rsc.org/en/content/articlepdf/2022/CY/D2CY00205A

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5. Cascade upgrading of γ-valerolactone to biofuels

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