Direct synthesis of phenol by novel [FeFe]-hydrogenase model complexes as catalysts of benzene hydroxylation with H2O2-Reference-Cited by-同舟云学术

Direct synthesis of phenol by novel [FeFe]-hydrogenase model complexes as catalysts of benzene hydroxylation with H2O2

Published:2017 Issue:5 Volume:7 Page:2934-2942
ISSN:2046-2069
Container-title:RSC Advances
language:en
Short-container-title:RSC Adv.

Author:

Zhang Xia¹²³⁴⁵,Zhang Tianyong¹²³⁴⁵,Li Bin¹²³⁴⁵^ORCID,Zhang Guanghui¹²³⁴⁵,Hai Li¹²³⁴⁵,Ma Xiaoyuan¹²³⁴⁵,Wu Wubin¹²³⁴⁵

Affiliation:

1. Tianjin Key Laboratory of Applied Catalysis Science and Technology

2. School of Chemical Engineering and Technology

3. Tianjin University

4. Tianjin 300354

5. China

Abstract

Compared the catalytic performance of complexes 1–3, the complex 2 has the highest phenol yield (24.6%) and phenol selectivity (92%), which has the highest electron densities of the catalytically active sites.

Funder

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemical Engineering,General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2017/RA/C6RA27831K

Reference48 articles.

1. Hybrid compounds of Schiff base Cu, Fe, Co complexes with molybdovanadophoric heteropolyacids: synthesis, characterization and their catalytic performance to hydroxylation of benzene with H2O2

2. Hydroxylation of benzene with oxygen and hydrogen over catalysts containing Group VIII metals and heteropoly compounds

3. Low temperature hydroxylation of benzene to phenol by hydrogen peroxide over Fe/activated carbon catalyst

4. Studies on vanadium catalyzed direct hydroxylation of aromatic hydrocarbons using hydrogen peroxide as oxidant

5. Direct Oxidation of Benzene to Phenol with Hydrogen Peroxide over a Modified Titanium Silicalite

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