Enhancing Cu–ligand interaction for efficient CO<sub>2</sub> reduction towards multi-carbon products-Reference-Cited by-同舟云学术

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Enhancing Cu–ligand interaction for efficient CO₂ reduction towards multi-carbon products

Published:2024 Issue:23 Volume:60 Page:3178-3181
ISSN:1359-7345
Container-title:Chemical Communications
language:en
Short-container-title:Chem. Commun.

Author:

Chen Jingyi¹,Fan Lei¹,Zhao Yilin¹^ORCID,Yang Haozhou¹^ORCID,Wang Di¹,Hu Bihao¹,Xi Shibo²,Wang Lei¹³^ORCID

Affiliation:

1. Department of Chemical and Biomolecular Engineering, National University of Singapore, 4 Engineering Drive 4, 117585, Singapore

2. Institute of Sustainability for Chemicals, Energy and Environment, A*STAR, 1 Pesek Road, Jurong Island, 627833, Singapore

3. Centre for Hydrogen Innovations, National University of Singapore, 4 Engineering Drive 4, 117585, Singapore

Abstract

Here, we report Cu-DAT (3,5-diamino-1,2,4-triazole) for efficient CO2 reduction. By optimizing the Cu/ligand cooperation, accelerated *CO adsorption and C–C coupling were achieved, demonstrating >80% C2+ products selectivity at 400 mA cm−2.

Funder

National Research Foundation Singapore

Agency for Science, Technology and Research

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/CC/D3CC05972C

Reference48 articles.

1. Strategies in catalysts and electrolyzer design for electrochemical CO 2 reduction toward C 2+ products

2. Electrochemical CO2 Reduction to Ethanol with Copper-Based Catalysts

3. Heterogeneous Electrocatalysts for CO2 Reduction

4. Effects of the Catalyst Dynamic Changes and Influence of the Reaction Environment on the Performance of Electrochemical CO 2 Reduction

5. Electrochemical CO2 Reduction: Classifying Cu Facets

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