Self-driven dual hydrogen production system based on a bifunctional single-atomic Rh catalyst

Author:

Peng Xianyun12,Mi Yuying2,Liu Xijun3ORCID,Sun Jiaqiang4ORCID,Qiu Yuan2,Zhang Shusheng5ORCID,Ke Xiaoxing6ORCID,Wang Xinzhong1,Luo Jun2ORCID

Affiliation:

1. Information Technology Research Institute, Shenzhen Institute of Information Technology, Shenzhen 518172, China

2. Institute for New Energy Materials & Low-Carbon Technologies, Tianjin Key Lab for Photoelectric Materials & Devices, School of Materials Science and Engineering, Tianjin University of Technology, Tianjin 300384, China

3. MOE Key Laboratory of New Processing Technology for Non-Ferrous Metals and Materials, Guangxi Key Laboratory of Processing for Non-Ferrous Metals and Featured Materials, School of Physical Science and Technology, Guangxi University, Nanning 530004, China

4. State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001, China

5. College of Chemistry, Zhengzhou University, Zhengzhou 450000, China

6. Beijing Key Laboratory of Microstructure and Properties of Solids, Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing 100124, China

Abstract

A self-powered dual hydrogen production system constructed by combining a Zn–H2 battery and an overall hydrazine splitting unit with Rh single atoms supported on oxygen-functionalized Ti3C2Ox bifunctional catalyst achieves a promising H2 generation rate of 45.77 mmol h−1.

Funder

National Natural Science Foundation of China

Science Fund for Distinguished Young Scholars of Tianjin

Guangdong Province Higher Vocational Colleges and Schools Pearl River Scholar Funded Scheme

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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