Carbonyl mediated fluorescence in aceno[n]helicenones and fluoreno[n]helicenes

Author:

Šámal Michal1,Sturm Ludmilla2,Banasiewicz Marzena3ORCID,Deperasinska Irena3ORCID,Kozankiewicz Boleslaw3ORCID,Morawski Olaf3ORCID,Nagata Yuuya4,Dechambenoit Pierre2,Bock Harald2ORCID,Rossel Amandine2,Buděšínský Miloš1,Boudier Anthony5ORCID,Jančařík Andrej2ORCID

Affiliation:

1. Institute of Organic Chemistry and Biochemistry of the Czech Academy of Sciences, 166 10 Prague 6, Czech Republic

2. Université de Bordeaux, CNRS, Centre de Recherche Paul Pascal, CRPP, UMR 5031, 33600 Pessac, France

3. Institute of Physics, Polish Academy of Sciences, Al. Lotników 32/46, 02-668 Warsaw, Poland

4. Japan Institute for Chemical Reaction Design and Discovery (WPI-ICReDD), Hokkaido University, Sapporo, Hokkaido 001-0021, Japan

5. Institut de Chimie et Biologie des Membranes et des Nanoobjets (CBMN), Université de Bordeaux-INP, UMR 5248, Allée St Hilaire, 33607, Pessac Cedex, France

Abstract

Carbo[n]helicenes are poor emitters with the emission peak in purple or blue region. Attaching an aryl-carbonyl group to the helical skeleton shifts the absorption and emission to the visible region and improves the fluorescence quantum yield.

Funder

Core Research for Evolutional Science and Technology

Université de Bordeaux

Centre National de la Recherche Scientifique

Exploratory Research for Advanced Technology

Ministry of Education, Culture, Sports, Science and Technology

Publisher

Royal Society of Chemistry (RSC)

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